Selected current-use pesticides (CUPs) in coastal and offshore sediments of Bohai and Yellow seas
Zhong, Guangcai1,2; Tang, Jianhui1; Xie, Zhiyong2; Mi, Wenying2; Chen, Yingjun1; Moeller, Axel2; Sturm, Renate2; Zhang, Gan3; Ebinghaus, Ralf2; Tang, JH (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China. jhtang@yic.ac.cn
发表期刊ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
ISSN0944-1344
2015-02-01
卷号22期号:3页码:1653-1661
关键词Current-use Pesticides Bohai Sea Yellow Sea Sediment
DOI10.1007/s11356-014-2648-7
产权排序[Zhong, Guangcai; Tang, Jianhui; Chen, Yingjun] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Zhong, Guangcai; Xie, Zhiyong; Mi, Wenying; Moeller, Axel; Sturm, Renate; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany; [Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要China is one of the largest producers, consumers, and traders for pesticides in the world. Currently, there are more than 600 pesticide-active substances registered in China, whereas few studies were conducted to improve our understanding of the occurrence and environmental impact of current-use pesticides (CUPs) in China's environment. In this work, 72 surface sediment samples were taken from the coastal and offshore of Bohai and Yellow seas and were analyzed for six CUPs (trifluralin, dacthal, quintozene, endosulfan, chlorpyrifos, and dicofol) and two metabolites (pentachloroanisole and endosulfan sulfate). Sediment samples were categorized as estuarine or near-shore sediments (Laizhou Bay, Taozi Bay, Sishili Bay, and Jiaozhou Bay) and offshore sediments. Trifluralin, alpha-endosulfan, endosulfan sulfate, chlorpyrifos, dicofol, and pentachloroanisole were detected in more than 60 % of the samples. Dicofol was the predominant compound with concentrations mostly higher than 100 pg/g dry weight (dw) with the highest concentration of 18,000 pg/g dw. Concentrations of other compounds were mainly below 100 pg/g dw. CUP levels were much lower than the sediment screening benchmark calculated. The highest levels of alpha-endosulfan, endosulfan sulfate, trifluralin, and chlorpyrifos existed at Laizhou Bay, whereas pentachloroanisole and dicofol had highest mean concentrations at Jiaozhou Bay. Generally, no correlation between pesticide concentrations and total organic carbon was observed either for offshore samples or for near-shore samples.; China is one of the largest producers, consumers, and traders for pesticides in the world. Currently, there are more than 600 pesticide-active substances registered in China, whereas few studies were conducted to improve our understanding of the occurrence and environmental impact of current-use pesticides (CUPs) in China's environment. In this work, 72 surface sediment samples were taken from the coastal and offshore of Bohai and Yellow seas and were analyzed for six CUPs (trifluralin, dacthal, quintozene, endosulfan, chlorpyrifos, and dicofol) and two metabolites (pentachloroanisole and endosulfan sulfate). Sediment samples were categorized as estuarine or near-shore sediments (Laizhou Bay, Taozi Bay, Sishili Bay, and Jiaozhou Bay) and offshore sediments. Trifluralin, alpha-endosulfan, endosulfan sulfate, chlorpyrifos, dicofol, and pentachloroanisole were detected in more than 60 % of the samples. Dicofol was the predominant compound with concentrations mostly higher than 100 pg/g dry weight (dw) with the highest concentration of 18,000 pg/g dw. Concentrations of other compounds were mainly below 100 pg/g dw. CUP levels were much lower than the sediment screening benchmark calculated. The highest levels of alpha-endosulfan, endosulfan sulfate, trifluralin, and chlorpyrifos existed at Laizhou Bay, whereas pentachloroanisole and dicofol had highest mean concentrations at Jiaozhou Bay. Generally, no correlation between pesticide concentrations and total organic carbon was observed either for offshore samples or for near-shore samples.
文章类型Article
资助机构Environmental Sciences & Ecology
收录类别SCI
语种英语
关键词[WOS]PERSISTENT ORGANIC POLLUTANTS ; EAST CHINA SEA ; ORGANOCHLORINE-PESTICIDES ; POLYCHLORINATED-BIPHENYLS ; ATMOSPHERIC DEPOSITION ; TEMPERATURE-DEPENDENCE ; AQUATIC ECOSYSTEMS ; AQUEOUS ENDOSULFAN ; SURFACE SEDIMENTS ; NORTH CHINA
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000348917400014
引用统计
被引频次:17[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/8659
专题中国科学院海岸带环境过程与生态修复重点实验室
通讯作者Tang, JH (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China. jhtang@yic.ac.cn
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
2.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
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GB/T 7714
Zhong, Guangcai,Tang, Jianhui,Xie, Zhiyong,et al. Selected current-use pesticides (CUPs) in coastal and offshore sediments of Bohai and Yellow seas[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2015,22(3):1653-1661.
APA Zhong, Guangcai.,Tang, Jianhui.,Xie, Zhiyong.,Mi, Wenying.,Chen, Yingjun.,...&Tang, JH .(2015).Selected current-use pesticides (CUPs) in coastal and offshore sediments of Bohai and Yellow seas.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,22(3),1653-1661.
MLA Zhong, Guangcai,et al."Selected current-use pesticides (CUPs) in coastal and offshore sediments of Bohai and Yellow seas".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH 22.3(2015):1653-1661.
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