Institutional Repository of Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences (KLCEP)
Fingerprint and weathering characteristics of crude oils after Dalian oil spill, China | |
Wang, Chuanyuan1; Chen, Bing2; Zhang, Baiyu2; He, Shijie3; Zhao, Mingming1 | |
发表期刊 | MARINE POLLUTION BULLETIN |
2013-06-15 | |
卷号 | 71期号:1-2页码:64-68 |
关键词 | Source Identification Natural Weathering Diagnostic Ratios Delta C-13 Dalian Oil Spill |
DOI | 10.1016/j.marpolbul.2013.03.034 |
产权排序 | 1. Key Laboratory of Coastal Zone Environment Processes and Ecological Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai 264003, China 2. Faculty of Engineering & Applied Science, Memorial University of Newfoundland, St. John’s, NL A1B 3X5, Canada 3. College of Geography and Planning, Ludong University, Yantai 264025, China |
通讯作者 | Wang CY, Key Laboratory of Coastal Zone Environment Processes and Ecological Remediation, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences, Yantai 264003, China. cywang@yic.ac.cn |
英文摘要 | In an attempt to analyze the chemical characterization of oil residues and examine the suitability of chemical fingerprinting methods in oil spill investigations, multiple parameters sensitive to both sources and degree of weathering were used to characterize oil residues from "7-16" Dalian oil spill, China. Oil residues collected 90 days to 120 days after the spill showed a weathering pattern where significant amounts of light to middle molecular weight normal alkanes were depleted with pristane and phytane as dominant peaks. Diagnostic ratios developed from n-alkane and selected isoprenoids (e.g. Pr/Ph, n-C-17/Pr, n-C-18/Ph, carbon preference index, LMW/HMW-alkanes ratio), all display obvious changes over weathering time, indicating that these ratios are not valid for oil source identification. Furthermore, the biomarker ratios of hopanes and steranes with relative standard deviations (RSDs) of 0.88-4.08% were useful for source identification even for severely weathered oil residues. In addition, RSD of delta C-13 values of individual n-alkanes in oil residue varied from 0.07% to 0.20%, which suggest that stable carbon isotope profile of n-alkanes can also be a useful tool for tracing the source of an oil spill. (C) 2013 Elsevier Ltd. All rights reserved. |
文章类型 | Article |
资助机构 | National Natural Science Foundation of China 40806048 ; Key Projects in the Yantai Science & Technology Pillar Program 2011060 ; Key Laboratory for Ecological Environment in Coastal Areas, State Oceanic Administration 200907 |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | CHEMICAL-CHARACTERIZATION ; ISOTOPIC COMPOSITION ; N-ALKANES ; IDENTIFICATION ; HYDROCARBONS ; RESIDUES ; EGYPT ; TOOL |
研究领域[WOS] | Environmental Sciences & Ecology ; Marine & Freshwater Biology |
WOS记录号 | WOS:000321088200021 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/6770 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室 |
作者单位 | 1.Chinese Acad Sci, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China 2.Mem Univ Newfoundland, Fac Engn & Appl Sci, St John, NF A1B 3X5, Canada 3.Ludong Univ, Coll Geog & Planning, Yantai 264025, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Chuanyuan,Chen, Bing,Zhang, Baiyu,et al. Fingerprint and weathering characteristics of crude oils after Dalian oil spill, China[J]. MARINE POLLUTION BULLETIN,2013,71(1-2):64-68. |
APA | Wang, Chuanyuan,Chen, Bing,Zhang, Baiyu,He, Shijie,&Zhao, Mingming.(2013).Fingerprint and weathering characteristics of crude oils after Dalian oil spill, China.MARINE POLLUTION BULLETIN,71(1-2),64-68. |
MLA | Wang, Chuanyuan,et al."Fingerprint and weathering characteristics of crude oils after Dalian oil spill, China".MARINE POLLUTION BULLETIN 71.1-2(2013):64-68. |
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