Pyrolysis Temperature-Dependent Changes in the Characteristics of Biochar-Borne Dissolved Organic Matter and Its Copper Binding Properties | |
Wei, J; Tu, C; Yuan, GD; Bi, DX; Wang, HL; Zhang, LJ; Theng, BKG | |
发表期刊 | BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY |
ISSN | 0007-4861 |
2019-07 | |
卷号 | 103期号:1 SI页码:169-174 |
关键词 | Biochar DOM EEM PARAFAC C K-NEXAFS Copper-binding |
研究领域 | Environmental Sciences ; Toxicology |
DOI | 10.1007/s00128-018-2392-7 |
产权排序 | [Wei, Jing; Tu, Chen; Bi, Dongxue] Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Wei, Jing; Tu, Chen; Bi, Dongxue] YICCAS, Shandong Prov Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China; [Yuan, Guodong] Zhaoqing Univ, Sch Environm & Chem Engn, Zhaoqing 526061, Peoples R China; [Wang, Hailong] Foshan Univ, Sch Environm & Chem Engn, Foshan 528000, Peoples R China; [Zhang, Lijuan] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China; [Theng, Benny K. G.] Landcare Res, Private Bag 11052, Palmerston North 4442, New Zealand |
作者部门 | 海岸带环境过程实验室 |
英文摘要 | The dissolved organic matter (DOM) samples from biochars produced from Jerusalem artichoke stalks by pyrolysis at 300, 500, and 700 degrees C were characterized using a combination of spectroscopic techniques. Additionally, the binding affinities (long K-M) and the complexation capacities (C-L) of the DOM samples with Cu(II) were calculated to assess their Cu binding properties. The biochar-borne DOM contained mainly humic-like components (C1-C3) with a small amount of a protein-like component (C4). As the charring temperature increased, the concentrations of released DOM decreased. The low temperature biochar-borne DOM was found to have more carboxyl groups than its high temperature counterparts, and thus it had larger C-L values. In contrast, the high temperature biochar-borne DOM had larger long K-M values. Low temperature biochars, if applied in a large quantity, would alter copper mobility in the environment because of their high DOM contents and large copper binding capacities. |
文章类型 | Article |
资助机构 | National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41501522] ; Chinese National Key Research and Development Program [2016YFD0200303, 2016YFE0106400] ; National High Technology Research and Development ProgramNational High Technology Research and Development Program of China [2012AA06A204-4] |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | CARBON ; FLUORESCENCE ; RELEASE ; PLANT ; SOIL ; IMMOBILIZATION ; DISSOLUTION ; INSIGHTS |
研究领域[WOS] | Environmental Sciences ; Toxicology |
WOS记录号 | WOS:000475543500027 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/24904 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 中国科学院海岸带环境过程与生态修复重点实验室_污染过程与控制实验室 |
作者单位 | 1.Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; 2.YICCAS, Shandong Prov Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China; 3.Zhaoqing Univ, Sch Environm & Chem Engn, Zhaoqing 526061, Peoples R China; 4.Foshan Univ, Sch Environm & Chem Engn, Foshan 528000, Peoples R China; 5.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China; 6.Landcare Res, Private Bag 11052, Palmerston North 4442, New Zealand |
推荐引用方式 GB/T 7714 | Wei, J,Tu, C,Yuan, GD,et al. Pyrolysis Temperature-Dependent Changes in the Characteristics of Biochar-Borne Dissolved Organic Matter and Its Copper Binding Properties[J]. BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY,2019,103(1 SI):169-174. |
APA | Wei, J.,Tu, C.,Yuan, GD.,Bi, DX.,Wang, HL.,...&Theng, BKG.(2019).Pyrolysis Temperature-Dependent Changes in the Characteristics of Biochar-Borne Dissolved Organic Matter and Its Copper Binding Properties.BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY,103(1 SI),169-174. |
MLA | Wei, J,et al."Pyrolysis Temperature-Dependent Changes in the Characteristics of Biochar-Borne Dissolved Organic Matter and Its Copper Binding Properties".BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY 103.1 SI(2019):169-174. |
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