| Emission factors and environmental implication of organic pollutants in PM emitted from various vessels in China | |
Zhang, Fan; Chen, Yingjun; Cui, Min; Feng, Yanli; Yang, Xin; Chen, Jianmin; Zhang, Yan; Gao, Huiwang; Tian, Chongguo ; Matthias, Volker; Liu, Huan
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| 发表期刊 | ATMOSPHERIC ENVIRONMENT
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| ISSN | 1352-2310 |
| 2019-03-01 | |
| 卷号 | 200页码:302-311 |
| 关键词 | Emission factor Organic pollutants PM Vessel Environmental implication |
| 研究领域 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| DOI | 10.1016/j.atmosenv.2018.12.006 |
| 产权排序 | [Zhang, Fan; Cui, Min] Tongji Univ, China Meteorol Adm, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 00092, Peoples R China; [Zhang, Fan; Cui, Min] Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 00092, Peoples R China; [Chen, Yingjun; Yang, Xin; Chen, Jianmin; Zhang, Yan] Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200092, Peoples R China; [Feng, Yanli] Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China; [Gao, Huiwang] Ocean Univ China, Minist Educ China, Key Lab Marine Environm & Ecol, Qingdao, Peoples R China; [Gao, Huiwang] Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao 266071, Peoples R China; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China; [Matthias, Volker] Helmholtz Zentrum Geesthacht, Inst Coastal Res, Max Planck Str 1, D-21502 Geesthacht, Germany; [Liu, Huan] Tsinghua Univ, Sch Environm, Key Joint Lab ESPC, Beijing 100084, Peoples R China |
| 作者部门 | 海岸带环境工程技术研究与发展中心 |
| 英文摘要 | Organic pollutants from ship exhaust have significant health and air quality impact in coastal areas; their profiles are also in urgent need. Studies on organic pollutants from ships are still rare, especially in China. Therefore, 21 PAHs and 29 n-alkanes in PM emitted from 15 ships with different types and fuels under different operating modes in China were tested in this study. The results showed that: (1) Identified organic matters accounted for 0.15%-23.3% of PM. Fuel-based emission factors (EFs) for Sigma 16PAHs ranged from 0.095 to 5.80 mg (kg fuel)(-1), with low-engine-power fishing boats and heavy fuel oil (HFO) training ship had higher values compared with light diesel vessels. EFs for Sigma n-alkanes ranged from 5.22 to 1589 mg (kg fuel)(-1), with low-engine-power fishing boats had higher values compared with other vessels. (2) The dominant PAHs were medium molecular weight components of Pyr, Flua, Phe, and Chr. N-alkanes from C15 to C33 accounted for more than 97% of the total n-alkanes. (3) Ratios of typical PAHs and n-alkanes parameters in this study showed typical diagnostic characteristics of oil combustion source. Profiles and diagnostic characteristics of PAHs together with n-alkanes could provide a more precise source apportionment result in the future. (4) Besides, PAHs in PM emitted from ships inferred non-ignorable health influence. |
| 文章类型 | Article |
| 资助机构 | Natural Science Foundation of China [41761134083, 41603090, 91744203, 41473091] ; National Research Program for Key Issues in Air Pollution Control [DQGG0201] ; Fundamental Research Funds for the Central Universities |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | POLYCYCLIC AROMATIC-HYDROCARBONS ; FINE PARTICULATE MATTER ; SHIP EMISSIONS ; SOURCE IDENTIFICATION ; SOURCE APPORTIONMENT ; EXHAUST EMISSIONS ; N-ALKANES ; DIAGNOSTIC RATIOS ; TRACE-METALS ; RIVER DELTA |
| 研究领域[WOS] | Environmental Sciences ; Meteorology & Atmospheric Sciences |
| WOS记录号 | WOS:000458225500028 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/24642 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心 中国科学院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Tongji Univ, China Meteorol Adm, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 00092, Peoples R China; 2.Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 00092, Peoples R China; 3.Fudan Univ, Dept Environm Sci & Engn, Shanghai Key Lab Atmospher Particle Pollut & Prev, Shanghai 200092, Peoples R China; 4.Shanghai Univ, Sch Environm & Chem Engn, Inst Environm Pollut & Hlth, Shanghai 200444, Peoples R China; 5.Ocean Univ China, Minist Educ China, Key Lab Marine Environm & Ecol, Qingdao, Peoples R China; 6.Qingdao Natl Lab Marine Sci & Technol, Lab Marine Ecol & Environm Sci, Qingdao 266071, Peoples R China; 7.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Shandong, Peoples R China; 8.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Max Planck Str 1, D-21502 Geesthacht, Germany; 9.Tsinghua Univ, Sch Environm, Key Joint Lab ESPC, Beijing 100084, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Fan,Chen, Yingjun,Cui, Min,et al. Emission factors and environmental implication of organic pollutants in PM emitted from various vessels in China[J]. ATMOSPHERIC ENVIRONMENT,2019,200:302-311. |
| APA | Zhang, Fan.,Chen, Yingjun.,Cui, Min.,Feng, Yanli.,Yang, Xin.,...&Liu, Huan.(2019).Emission factors and environmental implication of organic pollutants in PM emitted from various vessels in China.ATMOSPHERIC ENVIRONMENT,200,302-311. |
| MLA | Zhang, Fan,et al."Emission factors and environmental implication of organic pollutants in PM emitted from various vessels in China".ATMOSPHERIC ENVIRONMENT 200(2019):302-311. |
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