Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China
Liang, Xiaoxue; Tian, Chongguo; Zong, Zheng; Wang, Xiaoping; Jiang, Wanyanhan; Chen, Yingjun; Ma, Jianmin; Luo, Yongming; Li, Jun; Zhang, Gan
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2018-11
卷号242期号:B页码:1353-1361
关键词Source-sink relationship Heavy metals Arsenic Water exchange Bohai sea North Yellow sea
研究领域Environmental Sciences & Ecology
DOI10.1016/j.envpol.2018.08.011
产权排序[Liang, Xiaoxue; Jiang, Wanyanhan; Ma, Jianmin] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China; [Tian, Chongguo; Zong, Zheng; Luo, Yongming] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Zong, Zheng; Li, Jun; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Wang, Xiaoping] Ludong Univ, Yantai 264025, Peoples R China; [Chen, Yingjun] Tongji Univ, Coll Environm Sci & Engn, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 200092, Peoples R China; [Ma, Jianmin] Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
作者部门海岸带环境过程实验室
英文摘要This study conducted a field campaign to collect atmospheric deposition samples of heavy metals and arsenic, a metalloid element with typical chemical-physical characteristics (HMA), from 12 sampling sites and water samples from 37 rivers across the Bohai Sea (BS) and North Yellow Sea (NYS) in China. The HMA budgets in the BS and NYS were quantified by a budget model, which was developed based on the HMA inputs from atmospheric deposition and riverine discharge, sequestration to sediment, and interexchange among the BS's four subareas and the NYS. Statistical analyses of 76 deposition samples and 109 water concentration samples showed that atmospheric deposition was a main pathway of Pb entering the BS and NYS, whereas riverine discharge dominated the input of Cr, Cu, Zn, Cd, and As into the marine environment. Modeled results showed that the fractions of HMA in the water bodies compared with their total burdens were 86.6 +/- 4.55% in the Liaodong Bay, 60.5 +/- 10.5% in the Bohai Bay, 20.9 +/- 9.05% in the Laizhou Bay, 95.1 +/- 2.06% in the Central BS, and 94.3 +/- 1.93% in the NYS. The lowest fraction of HMA in the Laizhou Bay was attributed to high sedimentation rates and higher suspended particulate matter concentrations due to inputs from the Yellow River. The modeled 1-, 10- and 100- year mass budgets indicated that the Liaodong Bay in the north of the BS was a sink of HMA, the Bohai Bay and Laizhou Bay in the west and south of the BS acted as sources, and the Central BS and NYS were a transition area for most HMA. (C) 2018 Elsevier Ltd. All rights reserved.
文章类型Article
资助机构Strategic Priority Research Program of the CAS [XDA11020402] ; Natural Scientific Foundation of China [41471413]
收录类别SCI
语种英语
关键词[WOS]REGIONAL BACKGROUND SITE ; PEARL RIVER DELTA ; NORTH CHINA ; ATMOSPHERIC DEPOSITION ; SPATIAL-DISTRIBUTION ; LAIZHOU BAY ; CONTAMINATION ASSESSMENT ; PETROLEUM HYDROCARBON ; SURFACE SEDIMENTS ; RISK-ASSESSMENT
研究领域[WOS]Environmental Sciences
WOS记录号WOS:000446282600035
引用统计
被引频次:39[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/24560
专题中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China;
2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China;
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China;
4.Ludong Univ, Yantai 264025, Peoples R China;
5.Tongji Univ, Coll Environm Sci & Engn, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 200092, Peoples R China;
6.Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
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GB/T 7714
Liang, Xiaoxue,Tian, Chongguo,Zong, Zheng,et al. Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China[J]. ENVIRONMENTAL POLLUTION,2018,242(B):1353-1361.
APA Liang, Xiaoxue.,Tian, Chongguo.,Zong, Zheng.,Wang, Xiaoping.,Jiang, Wanyanhan.,...&Zhang, Gan.(2018).Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China.ENVIRONMENTAL POLLUTION,242(B),1353-1361.
MLA Liang, Xiaoxue,et al."Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China".ENVIRONMENTAL POLLUTION 242.B(2018):1353-1361.
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