Pyrolysis temperature-dependent changes in the characteristics of biochar-borne dissolved organic matter and its copper binding properties
Wei J; Tu C; Yuan GD; Bi DX; Wang HL; Zhang LJ; Theng BKG
发表期刊Bulletin of Environmental Contamination and Toxicology
ISSN0007-4861
2019
卷号103期号:1页码:169–174
关键词Biochar DOM EEM PARAFAC C K-NEXAFS Copper-binding
DOI10.1007/s00128-018-2392-7
产权排序1
通讯作者Yuan, Guodong(yuanguodong@zqu.edu.cn)
英文摘要The dissolved organic matter (DOM) samples from biochars produced from Jerusalem artichoke stalks by pyrolysis at 300, 500, and 700 degrees C were characterized using a combination of spectroscopic techniques. Additionally, the binding affinities (long K-M) and the complexation capacities (C-L) of the DOM samples with Cu(II) were calculated to assess their Cu binding properties. The biochar-borne DOM contained mainly humic-like components (C1-C3) with a small amount of a protein-like component (C4). As the charring temperature increased, the concentrations of released DOM decreased. The low temperature biochar-borne DOM was found to have more carboxyl groups than its high temperature counterparts, and thus it had larger C-L values. In contrast, the high temperature biochar-borne DOM had larger long K-M values. Low temperature biochars, if applied in a large quantity, would alter copper mobility in the environment because of their high DOM contents and large copper binding capacities.
资助机构National Natural Science Foundation of China ; Chinese National Key Research and Development Program ; National High Technology Research and Development Program
收录类别SCI
语种英语
关键词[WOS]CARBON ; FLUORESCENCE ; RELEASE ; PLANT ; SOIL ; IMMOBILIZATION ; DISSOLUTION ; INSIGHTS
研究领域[WOS]Environmental Sciences & Ecology ; Toxicology
WOS记录号WOS:000475543500027
引用统计
被引频次:57[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/24151
专题中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室
通讯作者Yuan GD
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GB/T 7714
Wei J,Tu C,Yuan GD,et al. Pyrolysis temperature-dependent changes in the characteristics of biochar-borne dissolved organic matter and its copper binding properties[J]. Bulletin of Environmental Contamination and Toxicology,2019,103(1):169–174.
APA Wei J.,Tu C.,Yuan GD.,Bi DX.,Wang HL.,...&Theng BKG.(2019).Pyrolysis temperature-dependent changes in the characteristics of biochar-borne dissolved organic matter and its copper binding properties.Bulletin of Environmental Contamination and Toxicology,103(1),169–174.
MLA Wei J,et al."Pyrolysis temperature-dependent changes in the characteristics of biochar-borne dissolved organic matter and its copper binding properties".Bulletin of Environmental Contamination and Toxicology 103.1(2019):169–174.
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