YIC-IR  > 中科院海岸带环境过程与生态修复重点实验室
Alternative and Legacy Perfluoroalkyl Substances: Differences between European and Chinese River/Estuary Systems
Heydebreck, F; Tang, JH; Xie, ZY; Ebinghaus, R; Heydebreck, F (reprint author), Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Dept Environm Chem, Max Planck Str 1, D-21502 Geesthacht, Schleswig Holst, Germany. franziska.heydebreck@hzg.de; jhtang@yic.ac.cn
2015-07-21
Source PublicationENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
Volume49Issue:14Pages:8386-8395
Contribution Rank[Heydebreck, Franziska; Xie, Zhiyong; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Dept Environm Chem, D-21502 Geesthacht, Schleswig Holst, Germany; [Heydebreck, Franziska] Univ Hamburg, Dept Chem, D-20146 Hamburg, Germany; [Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Shandong, Peoples R China
AbstractThe production and use of long-chain perfluoroalkyl substances (PFASs) must comply with national and international regulations. Driven by increasingly stringent regulations, their production has been outsourced to less regulated countries in Asia: In addition, the fluoropolymer industry started to use fluorinated alternatives, such as 2,3,3,3-tetrafluoro-2-(1,1,2,2,3,3,3-heptafluoropropoxy)propanoic acid (HFPO-DA). Between August 2013 and September 2014, we investigated the occurrence and distribution of HFPO-DA and legacy PFASs in surface waters of the following river/estuary systems: the Elbe and Rhine Rivers in Germany, the Rhine-Meuse delta in The Netherlands, and the Xiaoqing River in China. Distinct differences were revealed among the study areas; notably, the Chinese samples were highly polluted by an industrial point source discharging mainly perfluorooctanoic acid (PFOA). This particular point solute resulted in concentrations more than 6000 times higher than an industrial point source observed in the Scheur River, where HFPO-DA was the dominant compound with a concentration of 73.1 ng/L. Moreover, HFPO-DA was detected in all Samples along the coastline of the North Sea, indicating that the compound may be transported from the Rhine-Meuse delta into the German Bight via the water current. To the best of our knowledge, the fluorinated alternative, HFPO-DA, was detected for the first time in surface Waters of Germany and China.
Department中科院海岸带环境过程与生态修复重点实验室
DOI10.1021/acs.est.5b01648
Indexed BySCI
WOS KeywordPOLYFLUOROALKYL SUBSTANCES ; PHYSICOCHEMICAL PROPERTIES ; FLUORINATED ALTERNATIVES ; CARBOXYLIC-ACIDS ; LAIZHOU BAY ; ENVIRONMENT ; PRECURSORS ; TRANSPORT ; PFAAS ; WATER
SubtypeArticle
Language英语
WOS Research AreaEngineering ; Environmental Sciences & Ecology
WOS IDWOS:000358557900015
Citation statistics
Cited Times:82[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.yic.ac.cn/handle/133337/9278
Collection中科院海岸带环境过程与生态修复重点实验室
Corresponding AuthorHeydebreck, F (reprint author), Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Dept Environm Chem, Max Planck Str 1, D-21502 Geesthacht, Schleswig Holst, Germany. franziska.heydebreck@hzg.de; jhtang@yic.ac.cn
Recommended Citation
GB/T 7714
Heydebreck, F,Tang, JH,Xie, ZY,et al. Alternative and Legacy Perfluoroalkyl Substances: Differences between European and Chinese River/Estuary Systems[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2015,49(14):8386-8395.
APA Heydebreck, F,Tang, JH,Xie, ZY,Ebinghaus, R,Heydebreck, F ,&jhtang@yic.ac.cn.(2015).Alternative and Legacy Perfluoroalkyl Substances: Differences between European and Chinese River/Estuary Systems.ENVIRONMENTAL SCIENCE & TECHNOLOGY,49(14),8386-8395.
MLA Heydebreck, F,et al."Alternative and Legacy Perfluoroalkyl Substances: Differences between European and Chinese River/Estuary Systems".ENVIRONMENTAL SCIENCE & TECHNOLOGY 49.14(2015):8386-8395.
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