Institutional Repository of Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences (KLCEP)
| Perfluoroalkyl acids (PFAAs) in riverine and coastal sediments of Laizhou Bay, North China | |
Zhao, Zhen1,2,4; Tang, Jianhui1 ; Xie, Zhiyong2; Chen, Yingjun1; Pan, Xiaohui1; Zhong, Guangcai1,2; Sturm, Renate2; Zhang, Gan3; Ebinghaus, Ralf2
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| 发表期刊 | SCIENCE OF THE TOTAL ENVIRONMENT
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| ISSN | 0048-9697 |
| 2013-03-01 | |
| 卷号 | 447页码:415-423 |
| 关键词 | Polyfluoroalkyl Acids (Pfaas) Laizhou Bay Perfluorooctanoic Acid (Pfoa) Sediment Riverine Input |
| 产权排序 | [Zhao, Zhen; Tang, Jianhui; Chen, Yingjun; Pan, Xiaohui; Zhong, Guangcai] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China; [Zhao, Zhen; Xie, Zhiyong; Zhong, Guangcai; Sturm, Renate; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Dept Environm Chem, Geesthacht, Germany; [Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China; [Zhao, Zhen] Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 通讯作者 | Tang, JH (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China. jhtang@yic.ac.cn |
| 作者部门 | 中科院海岸带环境过程与生态修复重点实验室 |
| 英文摘要 | This study investigates the concentrations and distributions of perfluoroalkyl acids (PFAAs), including perfluoroalkyl carboxylic acids (PFCAs) and perfluoroalkane sulphonates (PFSAs), in surface sediments from Laizhou Bay and its adjacent rivers. Sigma PFAAs showed much higher levels in the river sediment (with a mean of 5.25 ng/g dw) than in the coastal sediment (with a mean of 0.76 ng/g dw). Perfluorooctanoic acid (PFOA) was the predominant compound, accounting for 50% to 97% of Sigma PFAA concentrations in 70% of the samples. The highest concentrations were detected in the Xiaoqing River, possibly due to the rapid development of the nearby fluorochemical industry. Hydrodynamics strongly influenced the distribution of PFAAs in Laizhou Bay. The hydrophilic property of shorter-chained PFAAs (C <= 8) allowed them to be transported to the inner bay via currents, to adsorb onto suspended sediment and then to be deposited. The Xiaoqing River showed the highest PFOA concentration (76.9 ng/g dw) among the bodies of sediment that had been studied worldwide, which might pose a potential threat for the benthic organisms of this river. (C) 2013 Elsevier B.V. All rights reserved.; This study investigates the concentrations and distributions of perfluoroalkyl acids (PFAAs), including perfluoroalkyl carboxylic acids (PFCAs) and perfluoroalkane sulphonates (PFSAs), in surface sediments from Laizhou Bay and its adjacent rivers. Sigma PFAAs showed much higher levels in the river sediment (with a mean of 5.25 ng/g dw) than in the coastal sediment (with a mean of 0.76 ng/g dw). Perfluorooctanoic acid (PFOA) was the predominant compound, accounting for 50% to 97% of Sigma PFAA concentrations in 70% of the samples. The highest concentrations were detected in the Xiaoqing River, possibly due to the rapid development of the nearby fluorochemical industry. Hydrodynamics strongly influenced the distribution of PFAAs in Laizhou Bay. The hydrophilic property of shorter-chained PFAAs (C <= 8) allowed them to be transported to the inner bay via currents, to adsorb onto suspended sediment and then to be deposited. The Xiaoqing River showed the highest PFOA concentration (76.9 ng/g dw) among the bodies of sediment that had been studied worldwide, which might pose a potential threat for the benthic organisms of this river. (C) 2013 Elsevier B.V. All rights reserved. |
| 文章类型 | Article |
| 资助机构 | Chinese Academy of Sciences Initiative Projects [KZCX2-EW-QN210, KZCX2-YW-Q07-04]; National Science Foundation of China [40903048]; Shandong Province Project [2007GG2QT06018] |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | PERFLUOROOCTANE SULFONATE PFOS ; PERSISTENT ORGANIC POLLUTANTS ; WATER TREATMENT PLANTS ; PERFLUORINATED COMPOUNDS ; ENVIRONMENTAL FATE ; BOHAI SEA ; CONTAMINANTS ; SUBSTANCES ; PERFLUOROCHEMICALS ; SURFACTANTS |
| 研究领域[WOS] | Environmental Sciences & Ecology |
| WOS记录号 | WOS:000317538100045 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/6640 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China 2.Helmholtz Zentrum Geesthacht, Ctr Mat & Coastal Res, Inst Coastal Res, Dept Environm Chem, Geesthacht, Germany 3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Zhen,Tang, Jianhui,Xie, Zhiyong,et al. Perfluoroalkyl acids (PFAAs) in riverine and coastal sediments of Laizhou Bay, North China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2013,447:415-423. |
| APA | Zhao, Zhen.,Tang, Jianhui.,Xie, Zhiyong.,Chen, Yingjun.,Pan, Xiaohui.,...&Ebinghaus, Ralf.(2013).Perfluoroalkyl acids (PFAAs) in riverine and coastal sediments of Laizhou Bay, North China.SCIENCE OF THE TOTAL ENVIRONMENT,447,415-423. |
| MLA | Zhao, Zhen,et al."Perfluoroalkyl acids (PFAAs) in riverine and coastal sediments of Laizhou Bay, North China".SCIENCE OF THE TOTAL ENVIRONMENT 447(2013):415-423. |
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