Levels, spatial distribution and sources of selected antibiotics in the East River (Dongjiang), South China
Zhang, Ruijie1,2,3; Zhang, Gan1,2; Tang, Jianhui1; Xu, Weihai4; Li, Jun2; Liu, Xiang2; Zou, Yongde5; Chen, Xiaoxiang5; Li, Xiangdong6
发表期刊AQUATIC ECOSYSTEM HEALTH & MANAGEMENT
ISSN1463-4988
2012
卷号15期号:2页码:210-218
关键词Pharmaceuticals Macrolides Sulfonamides Trimethoprim Pearl River Delta
产权排序[Zhang, Ruijie; Zhang, Gan; Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China; [Zhang, Ruijie; Zhang, Gan; Li, Jun; Liu, Xiang] Chinese Acad Sci, State Key Lab Organ Geochem, Guangzhou Inst Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Zhang, Ruijie] Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China; [Xu, Weihai] Chinese Acad Sci, S China Sea Inst Oceanol, Guangzhou 510301, Guangdong, Peoples R China; [Zou, Yongde; Chen, Xiaoxiang] Nanhai Entry Exit Inspect & Quarantine, Foshan 528200, Peoples R China; [Li, Xiangdong] Hong Kong Polytech Univ, Dept Civil & Struct Engn, Hong Kong, Hong Kong, Peoples R China
通讯作者Zhang, G (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China.,zhanggan@gig.ac.cn
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要Eleven selected antibiotics in the East River, South China, were measured using high performance liquid chromatography-electrospray ionization tandem mass spectrometry (HPLC-EI-MS-MS). Erythromycin, roxitromycin, azithromycin, clarithromycin, sulfadimidine, sulfamethoxazole, sulfadiazine and trimethoprim were detected with frequencies of more than 75%, and average concentrations ranging from 0.9 to 67.4 ng l(-1). The other three compounds' (sulfathiazole, sulfacetamide and spiramycin) concentrations were below detection limits. In general, the concentrations of sulfonamides and trimethoprim were higher than those of macrolides. The concentrations of macrolides showed a spatial distribution pattern of delta > lower reach > middle reach (or urban area > agriculture area), while sulfonamides and trimethoprim did not have a significant spatial pattern. Principal component analysis and comparison with wastewater were further used to explore source information of the antibiotics. The results suggested that macrolides in the East River were mainly associated with domestic sewage, while sulfonamides and trimethoprim may be more related to agriculture wastewater, especially livestock industrial wastewater. It is suggested that to ensure/improve the drinking water quality in the region, a better pollution control of livestock industry in the lower and middle reaches is of critical importance.; Eleven selected antibiotics in the East River, South China, were measured using high performance liquid chromatography-electrospray ionization tandem mass spectrometry (HPLC-EI-MS-MS). Erythromycin, roxitromycin, azithromycin, clarithromycin, sulfadimidine, sulfamethoxazole, sulfadiazine and trimethoprim were detected with frequencies of more than 75%, and average concentrations ranging from 0.9 to 67.4 ng l(-1). The other three compounds' (sulfathiazole, sulfacetamide and spiramycin) concentrations were below detection limits. In general, the concentrations of sulfonamides and trimethoprim were higher than those of macrolides. The concentrations of macrolides showed a spatial distribution pattern of delta > lower reach > middle reach (or urban area > agriculture area), while sulfonamides and trimethoprim did not have a significant spatial pattern. Principal component analysis and comparison with wastewater were further used to explore source information of the antibiotics. The results suggested that macrolides in the East River were mainly associated with domestic sewage, while sulfonamides and trimethoprim may be more related to agriculture wastewater, especially livestock industrial wastewater. It is suggested that to ensure/improve the drinking water quality in the region, a better pollution control of livestock industry in the lower and middle reaches is of critical importance.
文章类型Article
资助机构Chinese Academy of Sciences[KZCX2-YW-Q02-01]; Open Fund of the State Key Laboratory of Organic Geochemistry[SKLOG2008a04]; The Hong Kong Polytechnic University
收录类别SCI
语种英语
关键词[WOS]TANDEM MASS-SPECTROMETRY ; PEARL RIVER ; MULTIRESIDUE DETERMINATION ; TREATMENT PLANTS ; WATER ; PHARMACEUTICALS ; SURFACE ; FATE ; CHLORAMPHENICOL ; TRIMETHOPRIM
研究领域[WOS]Environmental Sciences & Ecology ; Marine & Freshwater Biology ; Water Resources
WOS记录号WOS:000306323300014
引用统计
被引频次:32[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/6010
专题中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
2.Chinese Acad Sci, State Key Lab Organ Geochem, Guangzhou Inst Geochem, Guangzhou 510640, Guangdong, Peoples R China
3.Chinese Acad Sci, Grad Univ, Beijing 100039, Peoples R China
4.Chinese Acad Sci, S China Sea Inst Oceanol, Guangzhou 510301, Guangdong, Peoples R China
5.Nanhai Entry Exit Inspect & Quarantine, Foshan 528200, Peoples R China
6.Hong Kong Polytech Univ, Dept Civil & Struct Engn, Hong Kong, Hong Kong, Peoples R China
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GB/T 7714
Zhang, Ruijie,Zhang, Gan,Tang, Jianhui,et al. Levels, spatial distribution and sources of selected antibiotics in the East River (Dongjiang), South China[J]. AQUATIC ECOSYSTEM HEALTH & MANAGEMENT,2012,15(2):210-218.
APA Zhang, Ruijie.,Zhang, Gan.,Tang, Jianhui.,Xu, Weihai.,Li, Jun.,...&Li, Xiangdong.(2012).Levels, spatial distribution and sources of selected antibiotics in the East River (Dongjiang), South China.AQUATIC ECOSYSTEM HEALTH & MANAGEMENT,15(2),210-218.
MLA Zhang, Ruijie,et al."Levels, spatial distribution and sources of selected antibiotics in the East River (Dongjiang), South China".AQUATIC ECOSYSTEM HEALTH & MANAGEMENT 15.2(2012):210-218.
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