PAHs in soils and estimated air soil exchange in the Pearl River Delta, South China
Liu, Guoqing1,2; Yu, Lili2,3; Li, Jun2; Liu, Xiang2; Zhang, Gan2,4
发表期刊ENVIRONMENTAL MONITORING AND ASSESSMENT
ISSN0167-6369
2011-02-01
卷号173期号:1-4页码:861-870
关键词Soil Pahs Air Soil Exchange Pearl River Delta China
产权排序[Liu, Guoqing] Shenzhen Univ, Inst Appl Nucl Technol, Shenzhen 518060, Peoples R China; [Liu, Guoqing; Yu, Lili; Li, Jun; Liu, Xiang; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Yu, Lili] Univ Wollongong, Sch Earth & Environm Sci, GeoQuEST Res Ctr, Wollongong, NSW 2522, Australia; [Zhang, Gan] Chinese Acad Sci, Yantai Inst Coastal Zone Sustainable Dev, Yantai 264003, Peoples R China
通讯作者Liu, GQ, Shenzhen Univ, Inst Appl Nucl Technol, Shenzhen 518060, Peoples R China.liugq@szu.edu.cn
英文摘要In this study, 74 soil samples collected from the Pearl River Delta were analyzed for polycyclic aromatic hydrocarbons (PAHs). The PAH mixture in the soils is mainly of low molecular weight compounds, with naphthalene (21.4%) and phenanthrene (21.8%) being dominant. Soil PAH levels from the Pearl River Delta are relatively low (28-711 ng/g, averaged 192 ng/g) compared to those from urban soils in temperate regions. The mean concentration of EPAHs generally decrease with increasing distance from the city center, with EPAHs of paddy soils > crop soil > natural soil. PAHs in the air were measured during a year-round sampling campaign using semipermeable membrane devices, and the transfer of chemicals between the soil and air compartments were estimated. Soil air fugacity quotient calculations showed a highly uncertain equilibrium position of PAHs, with net volatilization of naphthalene and fluorene, whereas net deposition of phenanthrene, fluoranthene, and pyrene, indicating a capacity for the air to supply the soil with more substances.; In this study, 74 soil samples collected from the Pearl River Delta were analyzed for polycyclic aromatic hydrocarbons (PAHs). The PAH mixture in the soils is mainly of low molecular weight compounds, with naphthalene (21.4%) and phenanthrene (21.8%) being dominant. Soil PAH levels from the Pearl River Delta are relatively low (28-711 ng/g, averaged 192 ng/g) compared to those from urban soils in temperate regions. The mean concentration of EPAHs generally decrease with increasing distance from the city center, with EPAHs of paddy soils > crop soil > natural soil. PAHs in the air were measured during a year-round sampling campaign using semipermeable membrane devices, and the transfer of chemicals between the soil and air compartments were estimated. Soil air fugacity quotient calculations showed a highly uncertain equilibrium position of PAHs, with net volatilization of naphthalene and fluorene, whereas net deposition of phenanthrene, fluoranthene, and pyrene, indicating a capacity for the air to supply the soil with more substances.
文章类型Article
收录类别SCI
语种英语
关键词[WOS]POLYCYCLIC AROMATIC-HYDROCARBONS ; SEMIVOLATILE ORGANIC-COMPOUNDS ; ORGANOCHLORINE PESTICIDES ; AGRICULTURAL SOIL ; UNITED-STATES ; SEWAGE-SLUDGE ; CONTAMINANTS ; GUANGZHOU ; MODEL ; ATMOSPHERE
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000287982000063
引用统计
被引频次:30[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/4921
专题中国科学院烟台海岸带研究所知识产出
作者单位1.Shenzhen Univ, Inst Appl Nucl Technol, Shenzhen 518060, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
3.Univ Wollongong, Sch Earth & Environm Sci, GeoQuEST Res Ctr, Wollongong, NSW 2522, Australia
4.Chinese Acad Sci, Yantai Inst Coastal Zone Sustainable Dev, Yantai 264003, Peoples R China
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Liu, Guoqing,Yu, Lili,Li, Jun,et al. PAHs in soils and estimated air soil exchange in the Pearl River Delta, South China[J]. ENVIRONMENTAL MONITORING AND ASSESSMENT,2011,173(1-4):861-870.
APA Liu, Guoqing,Yu, Lili,Li, Jun,Liu, Xiang,&Zhang, Gan.(2011).PAHs in soils and estimated air soil exchange in the Pearl River Delta, South China.ENVIRONMENTAL MONITORING AND ASSESSMENT,173(1-4),861-870.
MLA Liu, Guoqing,et al."PAHs in soils and estimated air soil exchange in the Pearl River Delta, South China".ENVIRONMENTAL MONITORING AND ASSESSMENT 173.1-4(2011):861-870.
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