Organophosphate Esters in Air, Snow, and Seawater in the North Atlantic and the Arctic

doi:10.1021/acs.est.7b01289

	Organophosphate Esters in Air, Snow, and Seawater in the North Atlantic and the Arctic
	Li, Jing 1,2; Xie, Zhiyong 1; Mi, Wenying 3; Lai, Senchao 4; Tian, Chongguo5 ; Emeis, Kay-Christian 1,2; Ebinghaus, Ralf 1
发表期刊	ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN	0013-936X
	2017-06-20
卷号	51 期号:12 页码:6887-6896
关键词	FLAME RETARDANTS ATMOSPHERIC PARTICLES ORGANIC-COMPOUNDS SURFACE WATERS DRY DEPOSITION PLASTICIZERS FATE TOXICITY EXPOSURE GERMANY
研究领域	Engineering, Environmental ; Environmental Sciences
DOI	10.1021/acs.est.7b01289
产权排序	[Li, Jing; Xie, Zhiyong; Emeis, Kay-Christian; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany; [Li, Jing; Emeis, Kay-Christian] Univ Hamburg, Sch Integrated Climate Syst Sci, D-20144 Hamburg, Germany; [Mi, Wenying] MINJIE Analyt Lab, D-21502 Geesthacht, Germany; [Lai, Senchao] South China Univ Technol, Sch Environm & Energy, Guangdong Prov Engn & Technol Res Ctr Environm Ri, Guangzhou 510006, Guangdong, Peoples R China; [Tian, Chongguo] Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
作者部门	海岸带环境过程实验室
英文摘要	The concentrations of eight organophosphate esters (OPEs) have been investigated in air, snow and seawater samples collected during the 'cruise of ARK-XXVIII/2 from sixth June to third July 2014 across the North Atlantic and the Arctic. The sum of gaseous and particle concentrations (Sigma OPE) ranged from 3S to 343 pg/m(3). The three chkirinated OPEs accounted for 88 +/- 5% of the Sigma OPE. The most abundant OPE was tris(2-chloroethyl) phosphate (TCEP), with concentrations ranging from 30 to 227 pg/m(3), followed by three major OPEs; such as tris(1-chloro,2-propyl) phosphate (TCPP, 0.8 to 82 pg/M-3), tri.'n-butyl phosphate (TnBP, 2 to 19 pg/m(3)), and tri-iso-butyi phosphate (TiBP, 0.3 to 14 pg/m(3)). The LOPE concentrations in snow and seawater ranged from 4356 to 10561 pg/L and from 348 to 8396 pg/L, respectively. The atmospheric particle-bound dry depositions of TCEP ranged from 2 to 12 ng/m(2)/day. The air seawater gas exchange fluxes were dominated by net volatilization from seawater to air for TCEP (mean, 146 239 ng/tri(2)/day), TCPP (mean, 1670 +/- 3031 ng/m(2)/day), TiBP (mean, 537 581 ng/m(2)/day) and TnBP (mean, 230 +/- 254 ng/m(2)/clay). This study highlighted that OPEs are subject to long-range transport via both air and seawater from the European continent and seas to the North Atlantic and the Arctic.
文章类型	Article
收录类别	SCI
语种	英语
关键词[WOS]	FLAME RETARDANTS ; ATMOSPHERIC PARTICLES ; ORGANIC-COMPOUNDS ; SURFACE WATERS ; DRY DEPOSITION ; PLASTICIZERS ; FATE ; TOXICITY ; EXPOSURE ; GERMANY
研究领域[WOS]	Engineering ; Environmental Sciences & Ecology
WOS记录号	WOS:000404087400029
引用统计	被引频次：129[WOS] [WOS记录] [WOS相关记录]
文献类型	期刊论文
条目标识符	http://ir.yic.ac.cn/handle/133337/22542
专题	中国科学院海岸带环境过程与生态修复重点实验室
作者单位	1.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany 2.Univ Hamburg, Sch Integrated Climate Syst Sci, D-20144 Hamburg, Germany 3.MINJIE Analyt Lab, D-21502 Geesthacht, Germany 4.South China Univ Technol, Sch Environm & Energy, Guangdong Prov Engn & Technol Res Ctr Environm Ri, Guangzhou 510006, Guangdong, Peoples R China 5.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
推荐引用方式 GB/T 7714	Li, Jing,Xie, Zhiyong,Mi, Wenying,et al. Organophosphate Esters in Air, Snow, and Seawater in the North Atlantic and the Arctic[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2017,51(12):6887-6896.
APA	Li, Jing.,Xie, Zhiyong.,Mi, Wenying.,Lai, Senchao.,Tian, Chongguo.,...&Ebinghaus, Ralf.(2017).Organophosphate Esters in Air, Snow, and Seawater in the North Atlantic and the Arctic.ENVIRONMENTAL SCIENCE & TECHNOLOGY,51(12),6887-6896.
MLA	Li, Jing,et al."Organophosphate Esters in Air, Snow, and Seawater in the North Atlantic and the Arctic".ENVIRONMENTAL SCIENCE & TECHNOLOGY 51.12(2017):6887-6896.