Occurrence and spatial distribution of organophosphate ester flame retardants and plasticizers in 40 rivers draining into the Bohai Sea, north China
Wang, Runmei1,3; Tang, Jianhui1; Xie, Zhiyong2; Mi, Wenying2; Chen, Yingjun1; Wolschke, Hendrik2; Tian, Chongguo1; Pan, Xiaohui1; Luo, Yongming1; Ebinghaus, Ralf2; Tang, JH (reprint author), Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China. jhtang@yic.ac.cn; zhiyong.xie@hzg.de
发表期刊ENVIRONMENTAL POLLUTION
ISSN0269-7491
2015-03-01
卷号198页码:172-178
关键词Organophosphate Ester Surface Water Riverine Flux The Bohai Sea
DOI10.1016/j.envpol.2014.12.037
产权排序[Wang, Runmei; Tang, Jianhui; Chen, Yingjun; Tian, Chongguo; Pan, Xiaohui; Luo, Yongming] Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China; [Xie, Zhiyong; Mi, Wenying; Wolschke, Hendrik; Ebinghaus, Ralf] Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany; [Wang, Runmei] Univ Chinese Acad Sci, Beijing 100049, Peoples R China
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要Organophosphate esters (OPEs) are alternatives to polybrominated diphenyl ethers, often used as flameretardants and plasticizers. There are few reports of OPEs in river water. This study focused on the occurrence and spatial distribution of 11 OPE congeners and one synthetic intermediate triphenylphosphine oxide (TPPO) in 40 major rivers entering into the Bohai Sea. Total OPEs ranged from 9.6 to 1549 ng L-1, with an average of 300 ng L-1. Tris(1-chloro-2-propyl) phosphate (TCPP) (4.6-921 ng mean: 186 ng L-1) and tris(2-choroethyl) phosphate (TCEP) (1.3-268 ng L-1, mean: 80.2 ng L-1) were the most abundant OPEs and their distribution patterns are similar, indicating the same source (r = 0.61, P < 0.05) and the influence of large production and consumption of chlorinated OPEs in the region. Priority should be given to TCPP, PCEP and TPPO due to their high concentrations in the rivers and potential threat to aquatic organisms. (C) 2015 Elsevier Ltd. All rights reserved.; Organophosphate esters (OPEs) are alternatives to polybrominated diphenyl ethers, often used as flameretardants and plasticizers. There are few reports of OPEs in river water. This study focused on the occurrence and spatial distribution of 11 OPE congeners and one synthetic intermediate triphenylphosphine oxide (TPPO) in 40 major rivers entering into the Bohai Sea. Total OPEs ranged from 9.6 to 1549 ng L-1, with an average of 300 ng L-1. Tris(1-chloro-2-propyl) phosphate (TCPP) (4.6-921 ng mean: 186 ng L-1) and tris(2-choroethyl) phosphate (TCEP) (1.3-268 ng L-1, mean: 80.2 ng L-1) were the most abundant OPEs and their distribution patterns are similar, indicating the same source (r = 0.61, P < 0.05) and the influence of large production and consumption of chlorinated OPEs in the region. Priority should be given to TCPP, PCEP and TPPO due to their high concentrations in the rivers and potential threat to aquatic organisms. (C) 2015 Elsevier Ltd. All rights reserved.
文章类型Article
资助机构Environmental Sciences & Ecology
收录类别SCI
语种英语
关键词[WOS]FRESH-WATER STREAMS ; SURFACE WATERS ; RISK-ASSESSMENT ; DAPHNIA-MAGNA ; FATE ; PHARMACEUTICALS ; TOXICITY ; GERMANY
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000350191600022
引用统计
被引频次:301[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/8647
专题中国科学院海岸带环境过程与生态修复重点实验室
通讯作者Tang, JH (reprint author), Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China. jhtang@yic.ac.cn; zhiyong.xie@hzg.de
作者单位1.Chinese Acad Sci, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
2.Helmholtz Zentrum Geesthacht, Inst Coastal Res, Ctr Mat & Coastal Res, D-21502 Geesthacht, Germany
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Wang, Runmei,Tang, Jianhui,Xie, Zhiyong,et al. Occurrence and spatial distribution of organophosphate ester flame retardants and plasticizers in 40 rivers draining into the Bohai Sea, north China[J]. ENVIRONMENTAL POLLUTION,2015,198:172-178.
APA Wang, Runmei.,Tang, Jianhui.,Xie, Zhiyong.,Mi, Wenying.,Chen, Yingjun.,...&zhiyong.xie@hzg.de.(2015).Occurrence and spatial distribution of organophosphate ester flame retardants and plasticizers in 40 rivers draining into the Bohai Sea, north China.ENVIRONMENTAL POLLUTION,198,172-178.
MLA Wang, Runmei,et al."Occurrence and spatial distribution of organophosphate ester flame retardants and plasticizers in 40 rivers draining into the Bohai Sea, north China".ENVIRONMENTAL POLLUTION 198(2015):172-178.
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