Institutional Repository of Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences (KLCEP)
Fabrication, characterization and evaluation of mesoporous activated carbons from agricultural waste: Jerusalem artichoke stalk as an example | |
Yu, Lei1,2,3; Tu, Chen2; Luo, Yongming1,2; Luo, YM (reprint author), Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China. ymluo@yic.ac.cn | |
发表期刊 | FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING |
ISSN | 2095-2201 |
2015-04-01 | |
卷号 | 9期号:2页码:206-215 |
关键词 | Mesoporous Activated Carbon Response Surface Methodology Adsorption Isotherm Agricultural Wastes |
DOI | 10.1007/s11783-014-0631-7 |
产权排序 | [Yu, Lei; Luo, Yongming] Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China; [Yu, Lei; Tu, Chen; Luo, Yongming] Chinese Acad Sci, Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc, Yantai 264003, Peoples R China; [Yu, Lei] Nanjing Forestry Univ, Dept Environm Engn, Nanjing 210037, Jiangsu, Peoples R China |
作者部门 | 中科院海岸带环境过程与生态修复重点实验室 |
英文摘要 | This work explores the feasibility of Jerusalem artichoke stem (JAS), an agricultural waste, as an alternative precursor for fabrication of mesoporous activated carbon (MAC) via conventional ZnCl2 activation. The as-prepared JAS-MACs were characterized by thermogravimetric, nitrogen gas adsorption isotherm and high resolution scanning electron microscopy analysis. The interacting effects of chemical dosage, activation temperature and time on the mesoporosity, mesopore volume and carbon yield were investigated, and further optimized by response surface methodology (RSM). The Brunauer-Emmett-Teller surface area, mesoporosity and mesopore volume of the JAS-MAC prepared under optimum condition were identified to be 1631 m(2)center dot g(-1), 90.16% and 1.11 cm(3)center dot g(-1), respectively. Compared with commercial activated carbons, this carbon exhibited a comparable monolayer adsorption capacity of 374.5 mg center dot g(-1) for Methylene Blue dye. The findings suggest that RSM could be an effective approach for optimizing the pore structure of fabricated activated carbons.; This work explores the feasibility of Jerusalem artichoke stem (JAS), an agricultural waste, as an alternative precursor for fabrication of mesoporous activated carbon (MAC) via conventional ZnCl2 activation. The as-prepared JAS-MACs were characterized by thermogravimetric, nitrogen gas adsorption isotherm and high resolution scanning electron microscopy analysis. The interacting effects of chemical dosage, activation temperature and time on the mesoporosity, mesopore volume and carbon yield were investigated, and further optimized by response surface methodology (RSM). The Brunauer-Emmett-Teller surface area, mesoporosity and mesopore volume of the JAS-MAC prepared under optimum condition were identified to be 1631 m(2)center dot g(-1), 90.16% and 1.11 cm(3)center dot g(-1), respectively. Compared with commercial activated carbons, this carbon exhibited a comparable monolayer adsorption capacity of 374.5 mg center dot g(-1) for Methylene Blue dye. The findings suggest that RSM could be an effective approach for optimizing the pore structure of fabricated activated carbons. |
文章类型 | Article |
资助机构 | Engineering ; Environmental Sciences & Ecology |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | RESPONSE-SURFACE METHODOLOGY ; ZINC-CHLORIDE ACTIVATION ; ADSORPTION CHARACTERISTICS ; CHEMICAL ACTIVATION ; AQUEOUS-SOLUTION ; PHOSPHORIC-ACID ; OPTIMIZATION ; KINETICS ; REMOVAL ; THERMODYNAMICS |
研究领域[WOS] | Engineering ; Environmental Sciences & Ecology |
WOS记录号 | WOS:000349909300004 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/8639 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室 |
通讯作者 | Luo, YM (reprint author), Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China. ymluo@yic.ac.cn |
作者单位 | 1.Chinese Acad Sci, Inst Soil Sci, Key Lab Soil Environm & Pollut Remediat, Nanjing 210008, Jiangsu, Peoples R China 2.Chinese Acad Sci, Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc, Yantai 264003, Peoples R China 3.Nanjing Forestry Univ, Dept Environm Engn, Nanjing 210037, Jiangsu, Peoples R China |
推荐引用方式 GB/T 7714 | Yu, Lei,Tu, Chen,Luo, Yongming,et al. Fabrication, characterization and evaluation of mesoporous activated carbons from agricultural waste: Jerusalem artichoke stalk as an example[J]. FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING,2015,9(2):206-215. |
APA | Yu, Lei,Tu, Chen,Luo, Yongming,&Luo, YM .(2015).Fabrication, characterization and evaluation of mesoporous activated carbons from agricultural waste: Jerusalem artichoke stalk as an example.FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING,9(2),206-215. |
MLA | Yu, Lei,et al."Fabrication, characterization and evaluation of mesoporous activated carbons from agricultural waste: Jerusalem artichoke stalk as an example".FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING 9.2(2015):206-215. |
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