Atmospheric emission inventory of cadmium from anthropogenic sources | |
Cheng, K.1,2; Tian, H. Z.1; Zhao, D.1; Lu, L.1; Wang, Y.1,3; Chen, J.1; Liu, X. G.1; Jia, W. X.1; Huang, Z.1; Tian, HZ (reprint author), Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China. hztian@bnu.edu.cn | |
发表期刊 | INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY |
ISSN | 1735-1472 |
2014-04-01 | |
卷号 | 11期号:3页码:605-616 |
关键词 | Anthropogenic Emissions Cadmium Coal Combustion Nonferrous Metals Smelting Spatial Distribution Uncertainty Analysis |
DOI | 10.1007/s13762-013-0206-3 |
产权排序 | [Cheng, K.; Tian, H. Z.; Zhao, D.; Lu, L.; Wang, Y.; Chen, J.; Liu, X. G.; Jia, W. X.; Huang, Z.] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China; [Cheng, K.] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China; [Wang, Y.] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China |
作者部门 | 海岸带生物学与生物资源利用所重点实验室 |
英文摘要 | To demonstrate the atmospheric emission characteristics of cadmium (Cd), which is considered an important contaminant to human health and environment, a comprehensive emission inventory of Cd has been established by applying the best available emission factors and activity data for the first time. This inventory covers major anthropogenic sources in China and a bottom-up approach is adopted to compile the inventory for the sources where possible. The total emissions of Cd are estimated at about 743.77 metric tons for the year 2009, of which the contributions of industrial processes and combustion sources are approximately 56.6 and 43.4 %, respectively. Nonferrous metals smelting including copper, lead, and zinc, ranks as the leading source accounting for about 40.6 % of the total. The high contribution results from the rapid growth of nonferrous metallurgical industry that reflects a new focus of Cd emission pollution in China. Cd emissions from coal combustion are estimated at approximately 273.69 metric tons, with a share of 36.8 %, in which industrial coal-burning sector is thought to be the primary source. Moreover, Cd emissions are spatially allocated onto grid cells with a resolution of 0.5A degrees A xA 0.5A degrees, indicating that the emissions are mainly distributed among the regions of eastern, central and southern China. In addition, the uncertainties in the inventory are quantified by using a Monte Carlo simulation, and the overall uncertainty falls within a range of -15 to 48 %. It implies that more field tests for industrial coal combustion and metals smelting process are very necessary.; To demonstrate the atmospheric emission characteristics of cadmium (Cd), which is considered an important contaminant to human health and environment, a comprehensive emission inventory of Cd has been established by applying the best available emission factors and activity data for the first time. This inventory covers major anthropogenic sources in China and a bottom-up approach is adopted to compile the inventory for the sources where possible. The total emissions of Cd are estimated at about 743.77 metric tons for the year 2009, of which the contributions of industrial processes and combustion sources are approximately 56.6 and 43.4 %, respectively. Nonferrous metals smelting including copper, lead, and zinc, ranks as the leading source accounting for about 40.6 % of the total. The high contribution results from the rapid growth of nonferrous metallurgical industry that reflects a new focus of Cd emission pollution in China. Cd emissions from coal combustion are estimated at approximately 273.69 metric tons, with a share of 36.8 %, in which industrial coal-burning sector is thought to be the primary source. Moreover, Cd emissions are spatially allocated onto grid cells with a resolution of 0.5A degrees A xA 0.5A degrees, indicating that the emissions are mainly distributed among the regions of eastern, central and southern China. In addition, the uncertainties in the inventory are quantified by using a Monte Carlo simulation, and the overall uncertainty falls within a range of -15 to 48 %. It implies that more field tests for industrial coal combustion and metals smelting process are very necessary. |
文章类型 | Article |
资助机构 | Environmental Sciences & Ecology |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | SPATIAL VARIATION CHARACTERISTICS ; CHINA ; UNCERTAINTY ; DEPOSITION ; METALS ; COAL ; CD ; PB ; CR |
研究领域[WOS] | Environmental Sciences & Ecology |
WOS记录号 | WOS:000333253100005 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/8557 |
专题 | 海岸带生物学与生物资源利用重点实验室_海岸带生物学与生物资源保护实验室 |
通讯作者 | Tian, HZ (reprint author), Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China. hztian@bnu.edu.cn |
作者单位 | 1.Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China 2.Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China |
推荐引用方式 GB/T 7714 | Cheng, K.,Tian, H. Z.,Zhao, D.,et al. Atmospheric emission inventory of cadmium from anthropogenic sources[J]. INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY,2014,11(3):605-616. |
APA | Cheng, K..,Tian, H. Z..,Zhao, D..,Lu, L..,Wang, Y..,...&Tian, HZ .(2014).Atmospheric emission inventory of cadmium from anthropogenic sources.INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY,11(3),605-616. |
MLA | Cheng, K.,et al."Atmospheric emission inventory of cadmium from anthropogenic sources".INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY 11.3(2014):605-616. |
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