Atmospheric emission inventory of cadmium from anthropogenic sources
Cheng, K.1,2; Tian, H. Z.1; Zhao, D.1; Lu, L.1; Wang, Y.1,3; Chen, J.1; Liu, X. G.1; Jia, W. X.1; Huang, Z.1; Tian, HZ (reprint author), Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China. hztian@bnu.edu.cn
发表期刊INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY
ISSN1735-1472
2014-04-01
卷号11期号:3页码:605-616
关键词Anthropogenic Emissions Cadmium Coal Combustion Nonferrous Metals Smelting Spatial Distribution Uncertainty Analysis
DOI10.1007/s13762-013-0206-3
产权排序[Cheng, K.; Tian, H. Z.; Zhao, D.; Lu, L.; Wang, Y.; Chen, J.; Liu, X. G.; Jia, W. X.; Huang, Z.] Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China; [Cheng, K.] Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China; [Wang, Y.] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
作者部门海岸带生物学与生物资源利用所重点实验室
英文摘要To demonstrate the atmospheric emission characteristics of cadmium (Cd), which is considered an important contaminant to human health and environment, a comprehensive emission inventory of Cd has been established by applying the best available emission factors and activity data for the first time. This inventory covers major anthropogenic sources in China and a bottom-up approach is adopted to compile the inventory for the sources where possible. The total emissions of Cd are estimated at about 743.77 metric tons for the year 2009, of which the contributions of industrial processes and combustion sources are approximately 56.6 and 43.4 %, respectively. Nonferrous metals smelting including copper, lead, and zinc, ranks as the leading source accounting for about 40.6 % of the total. The high contribution results from the rapid growth of nonferrous metallurgical industry that reflects a new focus of Cd emission pollution in China. Cd emissions from coal combustion are estimated at approximately 273.69 metric tons, with a share of 36.8 %, in which industrial coal-burning sector is thought to be the primary source. Moreover, Cd emissions are spatially allocated onto grid cells with a resolution of 0.5A degrees A xA 0.5A degrees, indicating that the emissions are mainly distributed among the regions of eastern, central and southern China. In addition, the uncertainties in the inventory are quantified by using a Monte Carlo simulation, and the overall uncertainty falls within a range of -15 to 48 %. It implies that more field tests for industrial coal combustion and metals smelting process are very necessary.; To demonstrate the atmospheric emission characteristics of cadmium (Cd), which is considered an important contaminant to human health and environment, a comprehensive emission inventory of Cd has been established by applying the best available emission factors and activity data for the first time. This inventory covers major anthropogenic sources in China and a bottom-up approach is adopted to compile the inventory for the sources where possible. The total emissions of Cd are estimated at about 743.77 metric tons for the year 2009, of which the contributions of industrial processes and combustion sources are approximately 56.6 and 43.4 %, respectively. Nonferrous metals smelting including copper, lead, and zinc, ranks as the leading source accounting for about 40.6 % of the total. The high contribution results from the rapid growth of nonferrous metallurgical industry that reflects a new focus of Cd emission pollution in China. Cd emissions from coal combustion are estimated at approximately 273.69 metric tons, with a share of 36.8 %, in which industrial coal-burning sector is thought to be the primary source. Moreover, Cd emissions are spatially allocated onto grid cells with a resolution of 0.5A degrees A xA 0.5A degrees, indicating that the emissions are mainly distributed among the regions of eastern, central and southern China. In addition, the uncertainties in the inventory are quantified by using a Monte Carlo simulation, and the overall uncertainty falls within a range of -15 to 48 %. It implies that more field tests for industrial coal combustion and metals smelting process are very necessary.
文章类型Article
资助机构Environmental Sciences & Ecology
收录类别SCI
语种英语
关键词[WOS]SPATIAL VARIATION CHARACTERISTICS ; CHINA ; UNCERTAINTY ; DEPOSITION ; METALS ; COAL ; CD ; PB ; CR
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000333253100005
引用统计
被引频次:65[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/8557
专题海岸带生物学与生物资源利用重点实验室_海岸带生物学与生物资源保护实验室
通讯作者Tian, HZ (reprint author), Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China. hztian@bnu.edu.cn
作者单位1.Beijing Normal Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100875, Peoples R China
2.Zhejiang Univ, State Key Lab Clean Energy Utilizat, Hangzhou 310027, Zhejiang, Peoples R China
3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai 264003, Peoples R China
推荐引用方式
GB/T 7714
Cheng, K.,Tian, H. Z.,Zhao, D.,et al. Atmospheric emission inventory of cadmium from anthropogenic sources[J]. INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY,2014,11(3):605-616.
APA Cheng, K..,Tian, H. Z..,Zhao, D..,Lu, L..,Wang, Y..,...&Tian, HZ .(2014).Atmospheric emission inventory of cadmium from anthropogenic sources.INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY,11(3),605-616.
MLA Cheng, K.,et al."Atmospheric emission inventory of cadmium from anthropogenic sources".INTERNATIONAL JOURNAL OF ENVIRONMENTAL SCIENCE AND TECHNOLOGY 11.3(2014):605-616.
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