Atmospheric polychlorinated naphthalenes (PCNs) in India and Pakistan
Xu, Yue1; Li, Jun1; Chakraborty, Paromita2; Syed, Jabir Hussain3; Malik, Riffat Naseem4; Wang, Yan1; Tian, Chongguo5,6; Luo, Chunling1; Zhang, Gan1; Jones, Kevin C.7
发表期刊SCIENCE OF THE TOTAL ENVIRONMENT
ISSN0048-9697
2014
卷号466页码:1030-1036
关键词Pcns India Pakistan Passive Air Sampler Puf
产权排序[Xu, Yue; Li, Jun; Wang, Yan; Luo, Chunling; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Chakraborty, Paromita] SRM Univ, SRM Res Inst, Kattankulathur, Tamil Nadu, India; [Syed, Jabir Hussain] Quaid I Azam Univ, Dept Plant Sci, Environm Biol Lab, Islamabad 45320, Pakistan; [Malik, Riffat Naseem] Quaid I Azam Univ, Dept Environm Sci, Environm Biol & Ecotoxicol Lab, Islamabad 45320, Pakistan; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Shandong, Peoples R China; [Tian, Chongguo] YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China; [Jones, Kevin C.] Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England
通讯作者Li, J (reprint author), Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China. junli@gig.ac.cn
英文摘要Polychlorinated naphthalenes (PCNs) are now under review by the Stockholm Convention as candidates for persistent organic pollutants (POPs) due to their persistence, toxicity, bioaccumulation, and long-range atmospheric transport. Data on PCN levels are sparse in South Asia. Atmospheric PCNs in India and Pakistan were monitored during the winter by polyurethane foam disk passive air samplers (PUF-PAS). The average concentrations were 29 pg/m(3) and 7.7 pg/m(3) in the Indian and Pakistani samples, respectively. Those concentration levels were relatively lower than the previously reported values in other Asian countries, but still considerably higher than in other sites in the world. Tri-CNs and tetra-CNs were the dominant homologues in the air, especially in India. Spatially, the PCNs were ubiquitous in the target areas, and local distribution was generally impacted by the proximity to potential sources. Major sources of PCNs in this study were the re-emission of Halowax and industrial thermal processes. Biomass burning influenced some sites in Pakistan. However, the enrichment of tri-CNs in Indian cities cannot be ascribed to either the signature of a specific source or the preferential volatilization and/or photodegradation in tropical areas. Despite this unclear issue in South Asia, the present study indicates that the potential health impact was generally comparable to that in non-urban sites worldwide. (C) 2013 Elsevier B.V. All rights reserved.; Polychlorinated naphthalenes (PCNs) are now under review by the Stockholm Convention as candidates for persistent organic pollutants (POPs) due to their persistence, toxicity, bioaccumulation, and long-range atmospheric transport. Data on PCN levels are sparse in South Asia. Atmospheric PCNs in India and Pakistan were monitored during the winter by polyurethane foam disk passive air samplers (PUF-PAS). The average concentrations were 29 pg/m(3) and 7.7 pg/m(3) in the Indian and Pakistani samples, respectively. Those concentration levels were relatively lower than the previously reported values in other Asian countries, but still considerably higher than in other sites in the world. Tri-CNs and tetra-CNs were the dominant homologues in the air, especially in India. Spatially, the PCNs were ubiquitous in the target areas, and local distribution was generally impacted by the proximity to potential sources. Major sources of PCNs in this study were the re-emission of Halowax and industrial thermal processes. Biomass burning influenced some sites in Pakistan. However, the enrichment of tri-CNs in Indian cities cannot be ascribed to either the signature of a specific source or the preferential volatilization and/or photodegradation in tropical areas. Despite this unclear issue in South Asia, the present study indicates that the potential health impact was generally comparable to that in non-urban sites worldwide. (C) 2013 Elsevier B.V. All rights reserved.
文章类型Article
资助机构Chinese Academy of Sciences [KZCX2-YW-GJ02]; Ministry of Environmental Protection [201209018]; Natural Science Foundation of China (NSFC) [41125014, 40821003]
收录类别SCI
语种英语
关键词[WOS]PASSIVE AIR SAMPLERS ; ORGANOCHLORINE PESTICIDES ; HALOWAX SERIES ; COPLANAR PCBS ; COMBUSTION ; DIOXINS
研究领域[WOS]Environmental Sciences & Ecology
WOS记录号WOS:000330491600109
引用统计
被引频次:30[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/6916
专题中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
2.SRM Univ, SRM Res Inst, Kattankulathur, Tamil Nadu, India
3.Quaid I Azam Univ, Dept Plant Sci, Environm Biol Lab, Islamabad 45320, Pakistan
4.Quaid I Azam Univ, Dept Environm Sci, Environm Biol & Ecotoxicol Lab, Islamabad 45320, Pakistan
5.Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Shandong, Peoples R China
6.YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China
7.Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England
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Xu, Yue,Li, Jun,Chakraborty, Paromita,et al. Atmospheric polychlorinated naphthalenes (PCNs) in India and Pakistan[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2014,466:1030-1036.
APA Xu, Yue.,Li, Jun.,Chakraborty, Paromita.,Syed, Jabir Hussain.,Malik, Riffat Naseem.,...&Jones, Kevin C..(2014).Atmospheric polychlorinated naphthalenes (PCNs) in India and Pakistan.SCIENCE OF THE TOTAL ENVIRONMENT,466,1030-1036.
MLA Xu, Yue,et al."Atmospheric polychlorinated naphthalenes (PCNs) in India and Pakistan".SCIENCE OF THE TOTAL ENVIRONMENT 466(2014):1030-1036.
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