Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China | |
Liao, Chunyang1; Lv, Jungang2; Fu, Jianjie2; Zhao, Zongshan2; Liu, Fang1; Xue, Qinzhao1; Jiang, Guibin2 | |
发表期刊 | INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH |
ISSN | 0960-3123 |
2012 | |
卷号 | 22期号:4页码:317-330 |
关键词 | E-waste Soil Pahs Pcbs Ocps Residue |
产权排序 | [Liao, Chunyang; Liu, Fang; Xue, Qinzhao] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China; [Lv, Jungang; Fu, Jianjie; Zhao, Zongshan; Jiang, Guibin] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China |
通讯作者 | Liao, CY (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China.,cyliao@yic.ac.cn |
英文摘要 | Surface soils collected from Taizhou, a typical e-waste recycling area in Southeast China, were analyzed for the residues of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs) by using microwave-assisted extraction and gas chromatography -mass spectrometry (GC-MS). The total concentrations of 16 PAHs in US EPA's priority list (Sigma PAHs), six indicator PCBs (Sigma PCBs), 15 OCPs widely used in China (Sigma OCPs) in soils ranged from 125 to 4737 ng/g (average: 854 ng/g), from not detected to 55.4 ng/g (3.16 ng/g), and from 47.9 to 820 ng/g (276 ng/g), respectively. Individual PAHs were ubiquitously found in soil samples with detected ratio of 96% and their residual levels were comparable with those of serious polluted sites. Principal component analysis in combination with diagnostic ratios suggested that the combustion of coal, wood, and plastic wastes that are closely associated with illegal and unsafe recycling operations of e-wastes was the main source of PAHs in this area. Compared with other polluted sites, the PCBs residues in soils were generally low except for those in the major recycling site. The residual levels of OCPs in this region were also relatively higher and hexachlorocyclohexane (HCH), dichlorodiphenyltrichloroethane (DDT) and its metabolite forms including dichlorodiphenyldichloroethane (DDD) and dichlorodiphenyldichloroethylene (DDE), hexachlorobenzene (HCB), and dicofol were dominant species. The composition analysis indicated that the HCHs residues in soils might originate from the application of lindane (pure gamma-HCH) and parts of DDTs possibly from the wide use of dicofol with high impurity of DDT compounds in this region.; Surface soils collected from Taizhou, a typical e-waste recycling area in Southeast China, were analyzed for the residues of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs), and organochlorine pesticides (OCPs) by using microwave-assisted extraction and gas chromatography -mass spectrometry (GC-MS). The total concentrations of 16 PAHs in US EPA's priority list (Sigma PAHs), six indicator PCBs (Sigma PCBs), 15 OCPs widely used in China (Sigma OCPs) in soils ranged from 125 to 4737 ng/g (average: 854 ng/g), from not detected to 55.4 ng/g (3.16 ng/g), and from 47.9 to 820 ng/g (276 ng/g), respectively. Individual PAHs were ubiquitously found in soil samples with detected ratio of 96% and their residual levels were comparable with those of serious polluted sites. Principal component analysis in combination with diagnostic ratios suggested that the combustion of coal, wood, and plastic wastes that are closely associated with illegal and unsafe recycling operations of e-wastes was the main source of PAHs in this area. Compared with other polluted sites, the PCBs residues in soils were generally low except for those in the major recycling site. The residual levels of OCPs in this region were also relatively higher and hexachlorocyclohexane (HCH), dichlorodiphenyltrichloroethane (DDT) and its metabolite forms including dichlorodiphenyldichloroethane (DDD) and dichlorodiphenyldichloroethylene (DDE), hexachlorobenzene (HCB), and dicofol were dominant species. The composition analysis indicated that the HCHs residues in soils might originate from the application of lindane (pure gamma-HCH) and parts of DDTs possibly from the wide use of dicofol with high impurity of DDT compounds in this region. |
文章类型 | Article |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | ZHEJIANG PROVINCE ; SOURCE APPORTIONMENT ; HEAVY-METALS ; HCH RESIDUES ; HUMAN HEALTH ; RIVER-BASIN ; EAST CHINA ; SEDIMENTS ; DDT ; CONTAMINATION |
研究领域[WOS] | Environmental Sciences & Ecology ; Public, Environmental & Occupational Health |
WOS记录号 | WOS:000306743500003 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/6191 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室_污染过程与控制实验室 中国科学院烟台海岸带研究所知识产出 |
作者单位 | 1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China 2.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China |
推荐引用方式 GB/T 7714 | Liao, Chunyang,Lv, Jungang,Fu, Jianjie,et al. Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China[J]. INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH,2012,22(4):317-330. |
APA | Liao, Chunyang.,Lv, Jungang.,Fu, Jianjie.,Zhao, Zongshan.,Liu, Fang.,...&Jiang, Guibin.(2012).Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China.INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH,22(4),317-330. |
MLA | Liao, Chunyang,et al."Occurrence and profiles of polycyclic aromatic hydrocarbons (PAHs), polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in soils from a typical e-waste recycling area in Southeast China".INTERNATIONAL JOURNAL OF ENVIRONMENTAL HEALTH RESEARCH 22.4(2012):317-330. |
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