Assessing Environmental Fate of beta-HCH in Asian Soil and Association with Environmental Factors
Xu, Yue1,2,3; Tian, Chongguo1,2; Ma, Jianmin4; Zhang, Gan3; Li, Yi-Fan4; Ming, Lili3; Li, Jun3; Chen, Yingjun1,2; Tang, Jianhui1,2
2012-09-04
发表期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
卷号46期号:17页码:9525-9532
产权排序[Xu, Yue; Tian, Chongguo; Chen, Yingjun; Tang, Jianhui] Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China; [Xu, Yue; Tian, Chongguo; Chen, Yingjun; Tang, Jianhui] YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China; [Xu, Yue; Zhang, Gan; Ming, Lili; Li, Jun] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; [Ma, Jianmin; Li, Yi-Fan] Environm Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
摘要Chinese Gridded Pesticide Emission and Residue Model was applied to simulate long-term environmental fate of beta-HCH in Asia spanning 1948-2009. The model captured well the spatiotemporal variation of beta-HCH soil concentrations across the model domain. beta-HCH use in different areas within the model domain was simulated respectively to assess the influence of the different sources of beta-HCH on its environment fate. A mass center of soil residue (MCSR) was introduced and used to explore environmental factors contributing to the spatiotemporal variation of beta-HCH soil residue. Results demonstrate that the primary emission dominates beta-HCH soil residues during the use of this pesticide. After phase-out of the pesticide in 1999, the change in beta-HCH soil residues has been associated with the Asian summer monsoon, featured by northward displacement of the MCSR. The displacement from several major sources in China and northeastern Asia shows a downward trend at a 95% confidence level, largely caused by environmental degradation and northward delivery of beta-HCH under cold condition in northern area. The MCSRs away from the India and southern and southeastern Asia sources show a rapid northward displacement at a 99% confidence level, featuring the cold trapping effect of the Tibetan Plateau.; Chinese Gridded Pesticide Emission and Residue Model was applied to simulate long-term environmental fate of beta-HCH in Asia spanning 1948-2009. The model captured well the spatiotemporal variation of beta-HCH soil concentrations across the model domain. beta-HCH use in different areas within the model domain was simulated respectively to assess the influence of the different sources of beta-HCH on its environment fate. A mass center of soil residue (MCSR) was introduced and used to explore environmental factors contributing to the spatiotemporal variation of beta-HCH soil residue. Results demonstrate that the primary emission dominates beta-HCH soil residues during the use of this pesticide. After phase-out of the pesticide in 1999, the change in beta-HCH soil residues has been associated with the Asian summer monsoon, featured by northward displacement of the MCSR. The displacement from several major sources in China and northeastern Asia shows a downward trend at a 95% confidence level, largely caused by environmental degradation and northward delivery of beta-HCH under cold condition in northern area. The MCSRs away from the India and southern and southeastern Asia sources show a rapid northward displacement at a 99% confidence level, featuring the cold trapping effect of the Tibetan Plateau.
通讯作者Tian, CG (reprint author), Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China.
关键词Polybrominated Diphenyl Ethers Persistent Organic Pollutants Organochlorine Pesticides Polychlorinated-biphenyls Tibetan Plateau Hexachlorocyclohexane Isomers Chinese Cities Alpha-hch Chemicals Inventories
作者部门中科院海岸带环境过程与生态修复重点实验室
学科领域Engineering ; Environmental Sciences & Ecology
项目资助者Chinese Academy of Sciences [KZCX2-YW-GJ02, KZCX2-YW-QN210]; Promotive Research Foundation for Excellent Young and Middle-Aged Scientists of Shandong Province [BS2012HZ028]; Natural Scientific Foundation of China [41101495, 41125014]
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收录类别SCI
关键词[WOS]POLYBROMINATED DIPHENYL ETHERS ; PERSISTENT ORGANIC POLLUTANTS ; ORGANOCHLORINE PESTICIDES ; POLYCHLORINATED-BIPHENYLS ; TIBETAN PLATEAU ; HEXACHLOROCYCLOHEXANE ISOMERS ; CHINESE CITIES ; ALPHA-HCH ; CHEMICALS ; INVENTORIES
文章类型Article
语种英语
资助项目Xu, Yue; Tian, Chongguo; Ma, Jianmin; Zhang, Gan; Li, Yi-Fan; Ming, Lili; Li, Jun; Chen, Yingjun; Tang, Jianhui
WOS研究方向Engineering ; Environmental Sciences & Ecology
WOS记录号WOS:000308260700038
引用统计
被引频次:10[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/5959
专题中科院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China
2.YICCAS, Shandong Prov Key Lab Coastal Zone Environm Proc, Yantai 264003, Shandong, Peoples R China
3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China
4.Environm Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
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Xu, Yue,Tian, Chongguo,Ma, Jianmin,et al. Assessing Environmental Fate of beta-HCH in Asian Soil and Association with Environmental Factors[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2012,46(17):9525-9532.
APA Xu, Yue.,Tian, Chongguo.,Ma, Jianmin.,Zhang, Gan.,Li, Yi-Fan.,...&Tang, Jianhui.(2012).Assessing Environmental Fate of beta-HCH in Asian Soil and Association with Environmental Factors.ENVIRONMENTAL SCIENCE & TECHNOLOGY,46(17),9525-9532.
MLA Xu, Yue,et al."Assessing Environmental Fate of beta-HCH in Asian Soil and Association with Environmental Factors".ENVIRONMENTAL SCIENCE & TECHNOLOGY 46.17(2012):9525-9532.
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