Institutional Repository of Key Laboratory of Coastal Zone Environmental Processes, Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences (KLCEP)
Kinetic study on the sorption and degradation of antibiotics in the estuarine water: an evaluation based on single and multiple reactions | |
Li, Jia1,2,3; Cui, Min1 | |
发表期刊 | ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH |
ISSN | 0944-1344 |
2020-07-24 | |
页码 | 11 |
关键词 | Antibiotics Kinetics Sorption Hydrolysis Photolysis Biodegradation Estuarine water |
DOI | 10.1007/s11356-020-10194-4 |
通讯作者 | Li, Jia(lijia3611@yzu.edu.cn) |
英文摘要 | It is important to study the fate and transport of antibiotics in aquatic environments to reveal their pollution status. The premise behind fate and transport studies is to evaluate the reaction processes of the target antibiotics. However, available research on the environmental behaviors of antibiotics in certain natural waters, such as estuarine water, is scarce. In this study, single reactions such as sorption, biodegradation, and photolysis and multiple degradation reactions of sulfamethoxazole (SMX), trimethoprim (TMP), and ciprofloxacin (CIP) in the estuarine water were studied. The sorption rates of the target antibiotics in the estuarine water-sediment system were very fast, and the sorption amounts varied among sediments and antibiotics. Hydrolysis did not contribute to the degradation of the target antibiotics. Biodegradation had a low contribution to the degradation of the target antibiotics in the estuarine water. In comparison, photolysis was the dominant degradation process for SMX, TMP, and CIP. The rates of photolysis of the tested antibiotics in the estuarine water were greater than those in pure water; thereby, indicating photolysis of these antibiotics was more prone to occur in the estuarine water. In the multiple degradation experiments, it was found that there may be synergistic effects between the single degradation processes. Thus, the aqueous concentrations of antibiotics decreased rapidly by sorption after entering the estuarine water and then decreased relatively slowly by photolysis and biodegradation. This study provides information for evaluating the environmental behaviors of antibiotics in estuarine environments. |
资助机构 | Shandong Key Laboratory of Coastal Environmental Processes, YICCAS ; Natural Science Foundation of the Jiangsu Higher Education Institutions of China |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | PERSONAL CARE PRODUCTS ; RESISTANCE GENES ; PHARMACEUTICALS ; SULFAMETHOXAZOLE ; ADSORPTION ; RIVER ; FATE ; SULFAMETHAZINE ; CIPROFLOXACIN ; MECHANISM |
研究领域[WOS] | Environmental Sciences & Ecology |
WOS记录号 | WOS:000551767400007 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/28590 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 |
通讯作者 | Li, Jia |
作者单位 | 1.Yangzhou Univ, Sch Environm Sci & Engn, Yangzhou 225127, Jiangsu, Peoples R China 2.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China 3.YICCAS, Shandong Key Lab Coastal Environm Proc, Yantai 264003, Peoples R China |
推荐引用方式 GB/T 7714 | Li, Jia,Cui, Min. Kinetic study on the sorption and degradation of antibiotics in the estuarine water: an evaluation based on single and multiple reactions[J]. ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,2020:11. |
APA | Li, Jia,&Cui, Min.(2020).Kinetic study on the sorption and degradation of antibiotics in the estuarine water: an evaluation based on single and multiple reactions.ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH,11. |
MLA | Li, Jia,et al."Kinetic study on the sorption and degradation of antibiotics in the estuarine water: an evaluation based on single and multiple reactions".ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH (2020):11. |
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