| Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers | |
Jiang, Ming1,2; Sheng, Yanqing1 ; Liu, Qunqun1,2; Wang, Wenjing1; Liu, Xiaozhu1,2
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| 发表期刊 | SCIENCE OF THE TOTAL ENVIRONMENT
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| ISSN | 0048-9697 |
| 2021-01-15 | |
| 卷号 | 752页码:11 |
| 关键词 | Coastal rivers Sediment Inorganic sulfur Organic sulfur Buffer capacity |
| DOI | 10.1016/j.scitotenv.2020.141829 |
| 通讯作者 | Sheng, Yanqing(yqsheng@yic.ac.cn) |
| 英文摘要 | Geochemical processes of sulfur (S) in river aquatic systems play a crucial role in environmental evolution. In this study, the distributions and sources of reduced inorganic sulfur (RIS) and organic sulfur (OS) in coastal river surface sediments were investigated. The results indicated that OS dominated total S (80%), and OS (i.e., humic acid sulfur, HAS; fulvic acid sulfur, FAS) correlated with the availability of labile organic matter (OM) and reactive iron (Fe). Terrigenous inputs and sulfurization contributed to the enrichment of FAS through the S reduction. Autochthonous biological inputs were potential sources of HAS from S oxidization. The X-ray photoelectron spectroscopy showed that the main sources of S in surface sediments were deposited as the form of organic ester-sulfate. Aquatic life could break S down further, producing reduced S compounds accumulated as thiols and RIS in anoxic sediments. RIS was dominated by acid volatile sulfur (AVS) and chromium (II)-reducible sulfur (CRS). Reactive Fe oxides were major control factors for the conversation from hydrogen sulfide (H2S) to AVS, whereas elemental sulfide (ES) controlled the conversion from AVS into CRS in coastal rivers. (C) 2020 Elsevier B.V. All rights reserved. |
| 资助机构 | Strategic Priority Research Program of the Chinese Academy of Sciences ; National Natural Science Foundation of China ; Key Project of Research and Development Plan of Yantai ; Key Research and Development Program of Shandong Province |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | BUFFERING CAPACITY ; SPATIAL-DISTRIBUTION ; REACTIVE IRON ; JIAOZHOU BAY ; HUMIC SULFUR ; PHOSPHORUS ; DIAGENESIS ; SULFIDE ; ACCUMULATION ; ENRICHMENT |
| 研究领域[WOS] | Environmental Sciences & Ecology |
| WOS记录号 | WOS:000588243900049 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/28288 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心 中国科学院海岸带环境过程与生态修复重点实验室 |
| 通讯作者 | Sheng, Yanqing |
| 作者单位 | 1.Chinese Acad Sci, Res Ctr Coastal Environm Engn Technol Shandong Pr, Yantai Inst Coastal Zone Res, Yantai, Peoples R China 2.Univ Chinese Acad Sci, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Jiang, Ming,Sheng, Yanqing,Liu, Qunqun,et al. Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,752:11. |
| APA | Jiang, Ming,Sheng, Yanqing,Liu, Qunqun,Wang, Wenjing,&Liu, Xiaozhu.(2021).Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers.SCIENCE OF THE TOTAL ENVIRONMENT,752,11. |
| MLA | Jiang, Ming,et al."Conversion mechanisms between organic sulfur and inorganic sulfur in surface sediments in coastal rivers".SCIENCE OF THE TOTAL ENVIRONMENT 752(2021):11. |
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