| Remediation and its biological responses of Cd contaminated sediments using biochar and minerals with nanoscale zero-valent iron loading | |
Liu, Qunqun; Sheng, Yanqing ; Wang, Wenjing; Li, Changyu; Zhao, Guoqiang
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| 发表期刊 | SCIENCE OF THE TOTAL ENVIRONMENT
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| ISSN | 0048-9697 |
| 2020-04-15 | |
| 卷号 | 713页码:136650 |
| 关键词 | DISSOLVED ORGANIC-MATTER EXTRACELLULAR POLYMERIC SUBSTANCES IN-SITU STABILIZATION MICROBIAL COMMUNITY METAL CONTAMINATION RIVER SEDIMENTS STRAW BIOCHAR PADDY SOILS CADMIUM IMMOBILIZATION |
| 研究领域 | Environmental Sciences |
| DOI | 10.1016/j.scitotenv.2020.136650 |
| 产权排序 | [Liu, Qunqun; Sheng, Yanqing; Wang, Wenjing; Li, Changyu; Zhao, Guoqiang] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn Technol Shandong Pr, Yantai, Peoples R China; [Liu, Qunqun; Li, Changyu; Zhao, Guoqiang] Univ Chinese Acad Sci, Beijing, Peoples R China |
| 通讯作者 | Sheng, Yanqing(yqsheng@yic.ac.cn) |
| 作者部门 | 海岸带环境工程技术研究与发展中心 |
| 英文摘要 | Remediation of Cd pollution in sediments is crucial for the safety of aquatic environments and human health. In this study, four effective, common, and low-cost remediation materials (zeolite, sepiolite, red mud (RM), and biochar (BC)) loaded with nanoscale zero-valent iron (nZVI) and themselves were employed to immobilize Cd in sediments. The effects of different materials on sediment properties, immobilization effectiveness, bacterial communities, enzyme activities, and dissolved organic matter (DOM) were investigated. Results showed that sediment properties were significantly changed by the addition of immobilization materials (P < 0.05). The geochemical fraction analysis showed that the labile Cd was partially transformed to the stable fraction after immobilization, with an 11-47% decrease in the acid-soluble fraction and a 50-1000% increase in the residual fraction. The Cd immobilization effectiveness peaked at the nZVI/RM and nZVI/BC treatments, and the Cd toxicity characteristic leaching procedure (TCLP) leachabiities decreased by 42% and 44%, respectively. The modified materials were more effective for immobilizing Cd than the raw materials owing to the presence of nZVI, and the Cd TCLP leachabilities with the modified materials decreased by 15%-22% compared with the raw material treatments. Immobilization-driven reduction of bioava liable Cd enhanced the richness and diversity of bacterial communities and enzyme activities. Moreover, the immobilization treatment promoted the Fe(III)-reducing process by increasing the Fe(III)-reducing bacteria (e.g. Geobacteraceae, Bacillus, and Clostridium), which are conducive to Cd immobilization. Additionally, the DOM composition presented more autogenetic characteristics in treated groups. BC (nZVI/BC) can be selected as the priority material for Cd immobilization in sediments due to higher immobilization effectiveness and lower adverse effects on sediments. (C) 2020 Elsevier B.V. All rights reserved. |
| 文章类型 | Article |
| 资助机构 | Chinese Academy of Sciences (CAS)Chinese Academy of Sciences [XDA23050203] ; National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41373100] ; Regional Key Project of STS of CAS [KFJ-STS-QYZX-057] ; Key Research and Development Program of Shandong Province [2019GSF109002] |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | DISSOLVED ORGANIC-MATTER ; EXTRACELLULAR POLYMERIC SUBSTANCES ; IN-SITU STABILIZATION ; MICROBIAL COMMUNITY ; METAL CONTAMINATION ; RIVER SEDIMENTS ; STRAW BIOCHAR ; PADDY SOILS ; CADMIUM ; IMMOBILIZATION |
| 研究领域[WOS] | Environmental Sciences & Ecology |
| WOS记录号 | WOS:000514544700118 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/25048 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心 中国科学院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn Technol Shandong Pr, Yantai, Peoples R China; 2.Univ Chinese Acad Sci, Beijing, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Qunqun,Sheng, Yanqing,Wang, Wenjing,et al. Remediation and its biological responses of Cd contaminated sediments using biochar and minerals with nanoscale zero-valent iron loading[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2020,713:136650. |
| APA | Liu, Qunqun,Sheng, Yanqing,Wang, Wenjing,Li, Changyu,&Zhao, Guoqiang.(2020).Remediation and its biological responses of Cd contaminated sediments using biochar and minerals with nanoscale zero-valent iron loading.SCIENCE OF THE TOTAL ENVIRONMENT,713,136650. |
| MLA | Liu, Qunqun,et al."Remediation and its biological responses of Cd contaminated sediments using biochar and minerals with nanoscale zero-valent iron loading".SCIENCE OF THE TOTAL ENVIRONMENT 713(2020):136650. |
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