| Atmospheric nitrous acid (HONO) at a rural coastal site in North China: Seasonal variations and effects of biomass burning | |
Gu, Rongrong; Zheng, Penggang; Chen, Tianshu; Dong, Can; Wang, Ya'nan; Liu, Yiming; Liu, Yuhong; Luo, Yuanyuan; Han, Guangxuan ; Wang, Xinfeng; Zhou, Xuehua; Wang, Tao; Wang, Wenxing; Xue, Likun
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| 发表期刊 | ATMOSPHERIC ENVIRONMENT
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| ISSN | 1352-2310 |
| 2020-05-15 | |
| 卷号 | 229页码:117429 |
| 关键词 | YELLOW-RIVER DELTA NITRIC-OXIDE URBAN ATMOSPHERE CHEMISTRY EMISSIONS NO2 PHOTOLYSIS SURFACES DIOXIDE NITRATE |
| 研究领域 | Environmental Sciences ; Meteorology & Atmospheric Sciences |
| DOI | 10.1016/j.atmosenv.2020.117429 |
| 产权排序 | [Gu, Rongrong; Zheng, Penggang; Chen, Tianshu; Dong, Can; Liu, Yuhong; Luo, Yuanyuan; Wang, Xinfeng; Zhou, Xuehua; Wang, Wenxing; Xue, Likun] Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China; [Gu, Rongrong; Wang, Ya'nan; Liu, Yiming; Wang, Tao] Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 99907, Peoples R China; [Han, Guangxuan] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China; [Xue, Likun] Jinan Inst Environm Sci, Jinan 250100, Peoples R China |
| 通讯作者 | Xue, Likun(xuelikun@sdu.edu.cn) |
| 作者部门 | 海岸带环境过程实验室 |
| 英文摘要 | Nitrous acid (HONO) plays a significant role in atmospheric chemistry due to its contribution to hydroxyl radical (OH). However, no scientific consensus has been achieved about the daytime HONO formation mechanisms. To identify the seasonal variations of HONO chemistry and the impacts of biomass burning (BB), we performed a two-phased field study in winter-spring and summer (covering a harvest season) in 2017 at a rural coastal site in North China. Though the mean HONO concentration in winter-spring (0.26 +/- 0.28 ppbv) was higher than in summer (0.17 + 0.19 ppbv), the maximum HONO concentrations were comparable (similar to 2 ppbv) in the two campaigns. Both the HONO/NOx ratio and nocturnal heterogeneous conversion efficiency of HONO (C-HONO) in summer were over twice of that in winter-spring. The daytime budget analysis also revealed that the strength of P(othe)r (i.e., the HONO sources apart from the reaction of OH + NO) in summer was double of that in winter-spring. BB affected the HONO concentration by enhancing the contribution of heterogeneous HONO production on the aerosol surface but weakening the role of photo-related HONO formation. HONO photolysis was a significant source of OH in both winter-spring and summer, and its contribution could be further enhanced during the BB episode in summer. Our study demonstrates the significant seasonal variations of HONO and the effects of BB, and suggests needs for more multi-season observations and considerations of BB, especially during the harvest time, in HONO research. |
| 文章类型 | Article |
| 资助机构 | National Natural Science Foundation of ChinaNational Natural Science Foundation of China [41675118, 91544213, 41505111] ; Hong Kong Research Grants CouncilHong Kong Research Grants Council [T24-504/17-N] ; Shandong Provincial Natural Science Foundation for Distinguished Young Scholars [ZR2019JQ09] ; Qilu Youth Talent Program of Shandong University ; Jiangsu Collaborative Innovation Center for Climate Change |
| 收录类别 | SCI |
| 语种 | 英语 |
| 关键词[WOS] | YELLOW-RIVER DELTA ; NITRIC-OXIDE ; URBAN ATMOSPHERE ; CHEMISTRY ; EMISSIONS ; NO2 ; PHOTOLYSIS ; SURFACES ; DIOXIDE ; NITRATE |
| 研究领域[WOS] | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| WOS记录号 | WOS:000530031600004 |
| 引用统计 | |
| 文献类型 | 期刊论文 |
| 条目标识符 | http://ir.yic.ac.cn/handle/133337/25032 |
| 专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 中国科学院海岸带环境过程与生态修复重点实验室 |
| 作者单位 | 1.Shandong Univ, Environm Res Inst, Qingdao 266237, Peoples R China; 2.Hong Kong Polytech Univ, Dept Civil & Environm Engn, Hong Kong 99907, Peoples R China; 3.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China; 4.Jinan Inst Environm Sci, Jinan 250100, Peoples R China |
| 推荐引用方式 GB/T 7714 | Gu, Rongrong,Zheng, Penggang,Chen, Tianshu,et al. Atmospheric nitrous acid (HONO) at a rural coastal site in North China: Seasonal variations and effects of biomass burning[J]. ATMOSPHERIC ENVIRONMENT,2020,229:117429. |
| APA | Gu, Rongrong.,Zheng, Penggang.,Chen, Tianshu.,Dong, Can.,Wang, Ya'nan.,...&Xue, Likun.(2020).Atmospheric nitrous acid (HONO) at a rural coastal site in North China: Seasonal variations and effects of biomass burning.ATMOSPHERIC ENVIRONMENT,229,117429. |
| MLA | Gu, Rongrong,et al."Atmospheric nitrous acid (HONO) at a rural coastal site in North China: Seasonal variations and effects of biomass burning".ATMOSPHERIC ENVIRONMENT 229(2020):117429. |
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