Simultaneous Removal of SO2 and NOX by a Combination of Red Mud and Coal Mine Drainage
Li, Changyu; Sheng, Yanqing; Sun, Xiangyu
发表期刊ENVIRONMENTAL ENGINEERING SCIENCE
ISSN1092-8758
2018
卷号36期号:4页码:444-452
关键词denitration desulfurization mine water red mud
研究领域Engineering ; Environmental Sciences & Ecology
DOI10.1089/ees.2018.0360
产权排序[Li, Changyu; Sheng, Yanqing; Sun, Xiangyu] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn Technol Shandong Pr, Chunhui Rd 17, Yantai 264003, Peoples R China; [Li, Changyu; Sun, Xiangyu] Univ Chinese Acad Sci, Coll Resources & Environm, Beijing, Peoples R China
通讯作者Sheng, Yanqing(yqsheng@yic.ac.cn)
作者部门海岸带环境工程技术研究与发展中心
英文摘要Simultaneous removal of sulfur dioxide (SO2) and nitrogen oxides (NOX) is an important research field in air pollution control. The combination application of red mud (RM) with coal mine drainage as absorbent in simultaneous desulfurization and denitrification is an innovative attempt. In this study, a series of bubbling and spray tower tests were conducted to improve desulfurization and denitration abilities. Effects of RM concentration, gas flow, liquid-gas ratio, and SO2 concentration were investigated in the test. Our results indicated that SO2 removal efficiency depends primarily on RM concentration, gas flow, and the liquid-gas ratio. In the denitration test, the denitration characteristics of the absorbent were not consistent with industrial requirements, but denitration ability could be improved by the addition of an oxidant. In addition, influence of interactions between SO2 and NOX was observed, and low concentrations of SO2 could enhance NOX absorption, whereas high SO2 concentrations inhibit NOX absorption. Meanwhile, NOX concentration has a negligible effect on SO2 removal. Under optimized conditions, such as with RM concentration of 12%, gas flow of 40 L/min, liquid-gas ratio of 20 L/m(3), absorbent renewal rate of 15%, and a sodium chlorite concentration of 1.9%, desulfurization efficiency is >99.0%, and denitration efficiency ranges from 45.0% to 47.0%. RM and mine water slurry show strong potential as a novel absorbent for the simultaneous removal of SO2 and NOX. This study provides a potential feasible technology for reusing RM and coal mine drainage with low cost instead of conventional method.
文章类型Article; Early Access
资助机构National Natural Science Foundation of China [41373100] ; Science and Technology Program for Public Wellbeing of Shandong Province [2013kjhm060308] ; CAS Key Technology Talent Program
收录类别SCI
语种英语
关键词[WOS]FLUE-GAS ; DESULFURIZATION ; ABSORPTION ; WATER ; COMBUSTION ; LIMESTONE ; SULFIDE ; ALKALI ; OXIDE
研究领域[WOS]Engineering, Environmental ; Environmental Sciences
WOS记录号WOS:000451674300001
引用统计
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/24580
专题中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境工程技术研究与发展中心
中国科学院海岸带环境过程与生态修复重点实验室
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Res Ctr Coastal Environm Engn Technol Shandong Pr, Chunhui Rd 17, Yantai 264003, Peoples R China;
2.Univ Chinese Acad Sci, Coll Resources & Environm, Beijing, Peoples R China
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GB/T 7714
Li, Changyu,Sheng, Yanqing,Sun, Xiangyu. Simultaneous Removal of SO2 and NOX by a Combination of Red Mud and Coal Mine Drainage[J]. ENVIRONMENTAL ENGINEERING SCIENCE,2018,36(4):444-452.
APA Li, Changyu,Sheng, Yanqing,&Sun, Xiangyu.(2018).Simultaneous Removal of SO2 and NOX by a Combination of Red Mud and Coal Mine Drainage.ENVIRONMENTAL ENGINEERING SCIENCE,36(4),444-452.
MLA Li, Changyu,et al."Simultaneous Removal of SO2 and NOX by a Combination of Red Mud and Coal Mine Drainage".ENVIRONMENTAL ENGINEERING SCIENCE 36.4(2018):444-452.
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