Emission factors of organic carbon and elemental carbon for residential coal and biomass fuels in China- A new database for 39 fuel-stove combinations | |
Sun, Jianzhong; Zhi, Guorui; Jin, Wenjing; Chen, Yingjun; Shen, Guofeng; Tian, Chongguo; Zhang, Yuzhe; Zong, Zheng; Cheng, Miaomiao; Zhang, Xinmin; Zhang, Yang; Liu, Chunyu; Lu, Jinkui; Wang, Hongzhao; Xiang, Jianmin; Tong, Litao; Zhang, Xi | |
发表期刊 | ATMOSPHERIC ENVIRONMENT |
ISSN | 1352-2310 |
2018-10 | |
卷号 | 190页码:241-248 |
关键词 | Household coal Biomass fuel OC EC EF |
研究领域 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
DOI | 10.1016/j.atmosenv.2018.07.032 |
产权排序 | [Sun, Jianzhong; Lu, Jinkui; Wang, Hongzhao; Xiang, Jianmin; Tong, Litao; Zhang, Xi] Shangrao Normal Univ, Sch Phys Educ, Shangrao 334001, Jiangxi, Peoples R China; [Zhi, Guorui; Jin, Wenjing; Zhang, Yuzhe; Cheng, Miaomiao; Zhang, Xinmin; Zhang, Yang; Liu, Chunyu] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China; [Chen, Yingjun] Tongji Univ, State Key Lab Pollut Control & Resources Reuse, Key Lab Cities Mitigat & Adaptat Climate Change, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China; [Shen, Guofeng] Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; [Zong, Zheng] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China |
作者部门 | 海岸带环境过程实验室 |
英文摘要 | In recent years many households in northern China's rural areas tend to furnish their houses with water-circulating piping system for heating, which entails mini-boiler stoves to heat water via raw coal chunk or biomass pellets. In this study, consistent efforts were made to obtain first-hand emission factors of organic carbon (EFOC) and elemental carbon (EFEC) for residential solid fuel combustion. A total of 39 fuel/stove combinations, covering seven coals (with different geological maturities), eleven biomass fuels, and five different stoves, were tested. The mean EFOC and EFEC were (4.29 +/- 2.33) and (4.43 +/- 2.18) g/kg for residential coal combustion, (2.16 +/- 4.47) and (0.42 +/- 1.01) g/kg for indoor biomass burning. The EFs for tested coal combustion display a "bell shape" with the maximum EF value occurring at bitumite of middle maturity. Coal briquetting in this study led to a significant decrease in EFEC but a notable increase in EFOC, which contradicted with the result from some of previous studies that coal briquetting always leads to relatively low emissions of both OC and EC. The inside reason deserves further clarification. Averaging over the two mini-boiler stoves shows that the introduction of mini-boiler stoves can reduce 5% and 10% of OC from anthracite and bitumite, respectively, and 47% and 53% of EC from anthracite and bitumite, respectively, suggesting that transfer from pure heating stoves to mini-boiler stoves seems unlikely to increase carbonaceous particle emissions, particularly EC. The more significant decline in EFEC than in EFOC indicates that the access to mini-boiler stove for winter heating is very likely to be both a clean air measure and a warming mitigation approach. Updated emission inventories in China for the year of 2014 showed that the OC and EC emissions were 338 Gg and 529 Gg, respectively, from residential coal combustion, and 557 Gg and 79 Gg, respectively, from household biomass burning. |
文章类型 | Article |
资助机构 | National Key RD Plan [2017YFC0213001] ; Special Project of Fundamental Research Funds of the Chinese Research Academy of Environmental Sciences [JY41373131] ; Doctoral Research Foundation of Shangrao Normal University [6000165] ; National Natural Science Foundation of China [41373131] ; Study of Comprehensive Scheme for Air Pollution Prevention and Control in Hebi [DQGG-05-24] |
收录类别 | SCI |
语种 | 英语 |
关键词[WOS] | POLYCYCLIC AROMATIC-HYDROCARBONS ; FINE PARTICULATE MATTER ; BROWN CARBON ; BLACK CARBON ; HOUSEHOLD STOVES ; LIGHT-ABSORPTION ; WOOD COMBUSTION ; AIR-POLLUTION ; PAH EMISSIONS ; RURAL CHINA |
研究领域[WOS] | Environmental Sciences ; Meteorology & Atmospheric Sciences |
WOS记录号 | WOS:000444659400024 |
引用统计 | |
文献类型 | 期刊论文 |
条目标识符 | http://ir.yic.ac.cn/handle/133337/24538 |
专题 | 中国科学院海岸带环境过程与生态修复重点实验室_海岸带环境过程实验室 中国科学院海岸带环境过程与生态修复重点实验室 |
作者单位 | 1.Shangrao Normal Univ, Sch Phys Educ, Shangrao 334001, Jiangxi, Peoples R China; 2.Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China; 3.Tongji Univ, State Key Lab Pollut Control & Resources Reuse, Key Lab Cities Mitigat & Adaptat Climate Change, Coll Environm Sci & Engn, Shanghai 200092, Peoples R China; 4.Peking Univ, Coll Urban & Environm Sci, Beijing 100871, Peoples R China; 5.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; 6.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China |
推荐引用方式 GB/T 7714 | Sun, Jianzhong,Zhi, Guorui,Jin, Wenjing,et al. Emission factors of organic carbon and elemental carbon for residential coal and biomass fuels in China- A new database for 39 fuel-stove combinations[J]. ATMOSPHERIC ENVIRONMENT,2018,190:241-248. |
APA | Sun, Jianzhong.,Zhi, Guorui.,Jin, Wenjing.,Chen, Yingjun.,Shen, Guofeng.,...&Zhang, Xi.(2018).Emission factors of organic carbon and elemental carbon for residential coal and biomass fuels in China- A new database for 39 fuel-stove combinations.ATMOSPHERIC ENVIRONMENT,190,241-248. |
MLA | Sun, Jianzhong,et al."Emission factors of organic carbon and elemental carbon for residential coal and biomass fuels in China- A new database for 39 fuel-stove combinations".ATMOSPHERIC ENVIRONMENT 190(2018):241-248. |
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