Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China
Huang, Tao; Zhang, Xiaodong; Ling, Zaili; Zhang, Leiming; Gao, Hong; Tian, Chongguo; Guo, Jiujiu; Zhao, Yuan; Wang, Li; Ma, Jianmin; Ma, JM (reprint author), Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China.
发表期刊ENVIRONMENTAL SCIENCE & TECHNOLOGY
ISSN0013-936X
2016-12-06
卷号50期号:23页码:12885-12893
DOI10.1021/acs.est.6b04835
产权排序[Huang, Tao; Zhang, Xiaodong; Ling, Zaili; Gao, Hong; Guo, Jiujiu; Zhao, Yuan; Wang, Li; Ma, Jianmin] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China; [Zhang, Leiming] Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada; [Tian, Chongguo] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China; [Ma, Jianmin] CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
作者部门中科院海岸带环境过程与生态修复重点实验室
英文摘要This study quantifies the influence of large-scale land-use change induced by the artificial Three-Northern Regions Shelter Forest (TNRSF) across northern China on the environmental cycling of organic chemicals. Atmospheric removal and long-term trends of two polycyclic aromatic hydrocarbon (PAH) species, phenanthrene (PHE) and benzo[a]pyrene (BaP), resulting from increasing vegetation coverage and soil organic carbon in the TNRSF over the last two decades were examined. Field sampling data and modeling result showed that the total atmospheric removal of PHE by TNRSF increased from 36.4 tons in 1990 to 76.8 tons in 2010, increasing at a rate of 5.6% yr(-1), and BaP from 2.2 to 4.5 tons, increasing at a rate of 5.2% yr(-1). Three model scenarios were designed to distinguish the effects of atmospheric emissions, and with and without TNRSF on the environmental fate of PAHs. Approximately 1-4% of PHE and BaP emitted in northern China were removed by the TNRSF during 1990-2010. Model simulations revealed that the TNRSF enhanced atmospheric removal of PHE by 29% and BaP by 53% compared with the simulation without the TNRSF, manifesting marked contributions of land-use change by the artificial TNRSF, the largest afforestation activity in human history, to the atmospheric removal of organic chemicals.
文章类型Article
资助机构National Natural Science Foundation of China(41503089 ; Natural Science Foundation of Gansu Province of China(1506RJZA212) ; 41371478 ; 41371453)
收录类别SCI
语种英语
关键词[WOS]PERSISTENT ORGANIC POLLUTANTS ; GLOBAL CLIMATE-CHANGE ; POLYCHLORINATED-BIPHENYLS ; ENVIRONMENTAL FATE ; BACKGROUND SOILS ; DRY DEPOSITION ; CARBON STOCKS ; VEGETATION ; TRANSPORT ; PCBS
研究领域[WOS]Engineering ; Environmental Sciences & Ecology
WOS记录号WOS:000389557100041
引用统计
被引频次:15[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.yic.ac.cn/handle/133337/19263
专题中国科学院海岸带环境过程与生态修复重点实验室
通讯作者Ma, JM (reprint author), Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China.
作者单位1.Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China
2.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
3.Environm & Climate Change Canada, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Zone Environm Proc & Ecol Remedia, Yantai 264003, Peoples R China
5.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
推荐引用方式
GB/T 7714
Huang, Tao,Zhang, Xiaodong,Ling, Zaili,et al. Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China[J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY,2016,50(23):12885-12893.
APA Huang, Tao.,Zhang, Xiaodong.,Ling, Zaili.,Zhang, Leiming.,Gao, Hong.,...&Ma, JM .(2016).Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China.ENVIRONMENTAL SCIENCE & TECHNOLOGY,50(23),12885-12893.
MLA Huang, Tao,et al."Impacts of Large-Scale Land-Use Change on the Uptake of Polycyclic Aromatic Hydrocarbons in the Artificial Three Northern Regions Shelter Forest Across Northern China".ENVIRONMENTAL SCIENCE & TECHNOLOGY 50.23(2016):12885-12893.
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